Coherent Control Spectroscopy of Electronic and Nuclear Dynamics- [electronic resource]
Coherent Control Spectroscopy of Electronic and Nuclear Dynamics- [electronic resource]
- 자료유형
- 학위논문파일 국외
- 최종처리일시
- 20240214101519
- ISBN
- 9798380152785
- DDC
- 539
- 저자명
- Kaufman, Brian.
- 서명/저자
- Coherent Control Spectroscopy of Electronic and Nuclear Dynamics - [electronic resource]
- 발행사항
- [S.l.]: : State University of New York at Stony Brook., 2023
- 발행사항
- Ann Arbor : : ProQuest Dissertations & Theses,, 2023
- 형태사항
- 1 online resource(204 p.)
- 주기사항
- Source: Dissertations Abstracts International, Volume: 85-02, Section: B.
- 주기사항
- Advisor: Weinacht, Thomas C.
- 학위논문주기
- Thesis (Ph.D.)--State University of New York at Stony Brook, 2023.
- 사용제한주기
- This item must not be sold to any third party vendors.
- 초록/해제
- 요약Coherent control spectroscopy uses shaped or coherent light to manipulate and measure the quantum dynamics of electrons and nuclei in molecules. By shaping the amplitude and phase of laser pulses, one can tailor the initial wave function and influence the subsequent dynamics. This technique can be used to study various aspects of molecular motion, such as non-adiabatic dynamics (coupled motion of electrons and nuclei) and electronic coherence, both of which play an extremely important role in the photophysics of most molecules. In this thesis, I discuss the development of a specially designed ultrafast optical pulse shaper to generate and arbitrarily shape 5 fs pulses to study such molecular dynamics using a multiphoton driven version of time-resolved photoelectron spectroscopy (TR-PES). The ability to arbitrarily shape these laser pulses offers a vast toolbox of techniques that go beyond typical pump-probe measurements. The experiments described in this thesis provide a road map for a broad range of studies that follow and control electronic and nuclear dynamics using shaped laser pulses.
- 일반주제명
- Molecular physics.
- 일반주제명
- Atomic physics.
- 일반주제명
- Optics.
- 키워드
- Quantum dynamics
- 키워드
- Electrons
- 키워드
- Wave function
- 기타저자
- State University of New York at Stony Brook Physics
- 기본자료저록
- Dissertations Abstracts International. 85-02B.
- 기본자료저록
- Dissertation Abstract International
- 전자적 위치 및 접속
- 로그인 후 원문을 볼 수 있습니다.