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A Fractal Landscape Dynamics Approach to Understanding Particle Motion in Soft Jammed Materials
A Fractal Landscape Dynamics Approach to Understanding Particle Motion in Soft Jammed Mate...
A Fractal Landscape Dynamics Approach to Understanding Particle Motion in Soft Jammed Materials

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자료유형  
 학위논문 서양
최종처리일시  
20250211151059
ISBN  
9798382834559
DDC  
660
저자명  
Rodriguez-Cruz, Clary.
서명/저자  
A Fractal Landscape Dynamics Approach to Understanding Particle Motion in Soft Jammed Materials
발행사항  
[Sl] : University of Pennsylvania, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
116 p
주기사항  
Source: Dissertations Abstracts International, Volume: 85-12, Section: B.
주기사항  
Advisor: Crocker, John C.
학위논문주기  
Thesis (Ph.D.)--University of Pennsylvania, 2024.
초록/해제  
요약Soft jammed materials are disordered viscoelastic solids, composed of densely packed particles, that are commonly found both in the natural world and in a wide range of manufactured products. Their applications are widespread across various industries and technologies, including food, pharmaceuticals, agriculture and cosmetics. Understanding the fundamental physics and mathematics behind their highly complex particle motion and distinct response to external stress is essential for their improved design and stability, as well as the development of new materials with unique mechanical properties. Further, it is crucial for the development of theoretical models that better describe the complex interactions and dynamics of these materials. This thesis is centered around the observation that soft jammed materials exhibit fractal landscape dynamics, where the particles' motion is not merely random but follows patterns influenced by the system's underlying fractal energy landscape. Through experimental observations, theoretical models, and numerical simulations of ripening dense emulsions and foams, this work reveals two major findings. First, it demonstrates the numerical relationships between energy landscape geometry, microscopic particle dynamics, and macroscopic rheology through a novel high-dimensional approach. Second, it introduces a simplistic random walk model that generates fractal paths with specified dimensions, successfully reflecting the complex individual particle dynamics in a ripening foam after fitting to the data. This finding affirms the presence of fractal landscape dynamics as an explanation for behaviors such as non-Gaussian particle displacements, intermittent rearrangement events, and power-law rheology. Further exploration within this work extends the high-dimensional analysis framework to the dynamics of stock market prices, drawing an intriguing parallel between the motion of individual stocks and emulsion droplets. Lastly, the machine-learning metric of 'softness' is explored as a method to predict particle rearrangements in a ripening foam, showing that simply a particle's number of neighbors achieves a surprisingly high prediction accuracy. This thesis not only enhances our understanding of soft jammed materials but also opens new avenues for applying fractal landscape dynamics across different materials and research fields.
일반주제명  
Chemical engineering
일반주제명  
Energy
일반주제명  
Materials science
일반주제명  
Computational chemistry
일반주제명  
Particle physics
키워드  
Dense emulsion
키워드  
Energy landscape
키워드  
Fractal landscape dynamics
키워드  
Jammed materials
키워드  
Ripening foam
기타저자  
University of Pennsylvania Chemical and Biomolecular Engineering
기본자료저록  
Dissertations Abstracts International. 85-12B.
전자적 위치 및 접속  
로그인 후 원문을 볼 수 있습니다.

MARC

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■1001  ▼aRodriguez-Cruz,  Clary.
■24512▼aA  Fractal  Landscape  Dynamics  Approach  to  Understanding  Particle  Motion  in  Soft  Jammed  Materials
■260    ▼a[Sl]▼bUniversity  of  Pennsylvania▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a116  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  85-12,  Section:  B.
■500    ▼aAdvisor:  Crocker,  John  C.
■5021  ▼aThesis  (Ph.D.)--University  of  Pennsylvania,  2024.
■520    ▼aSoft  jammed  materials  are  disordered  viscoelastic  solids,  composed  of  densely  packed  particles,  that  are  commonly  found  both  in  the  natural  world  and  in  a  wide  range  of  manufactured  products.  Their  applications  are  widespread  across  various  industries  and  technologies,  including  food,  pharmaceuticals,  agriculture  and  cosmetics.  Understanding  the  fundamental  physics  and  mathematics  behind  their  highly  complex  particle  motion  and  distinct  response  to  external  stress  is  essential  for  their  improved  design  and  stability,  as  well  as  the  development  of  new  materials  with  unique  mechanical  properties.  Further,  it  is  crucial  for  the  development  of  theoretical  models  that  better  describe  the  complex  interactions  and  dynamics  of  these  materials.  This  thesis  is  centered  around  the  observation  that  soft  jammed  materials  exhibit  fractal  landscape  dynamics,  where  the  particles'  motion  is  not  merely  random  but  follows  patterns  influenced  by  the  system's  underlying  fractal  energy  landscape.  Through  experimental  observations,  theoretical  models,  and  numerical  simulations  of  ripening  dense  emulsions  and  foams,  this  work  reveals  two  major  findings.  First,  it  demonstrates  the  numerical  relationships  between  energy  landscape  geometry,  microscopic  particle  dynamics,  and  macroscopic  rheology  through  a  novel  high-dimensional  approach.  Second,  it  introduces  a  simplistic  random  walk  model  that  generates  fractal  paths  with  specified  dimensions,  successfully  reflecting  the  complex  individual  particle  dynamics  in  a  ripening  foam  after  fitting  to  the  data.  This  finding  affirms  the  presence  of  fractal  landscape  dynamics  as  an  explanation  for  behaviors  such  as  non-Gaussian  particle  displacements,  intermittent  rearrangement  events,  and  power-law  rheology.  Further  exploration  within  this  work  extends  the  high-dimensional  analysis  framework  to  the  dynamics  of  stock  market  prices,  drawing  an  intriguing  parallel  between  the  motion  of  individual  stocks  and  emulsion  droplets.  Lastly,  the  machine-learning  metric  of  'softness'  is  explored  as  a  method  to  predict  particle  rearrangements  in  a  ripening  foam,  showing  that  simply  a  particle's  number  of  neighbors  achieves  a  surprisingly  high  prediction  accuracy.  This  thesis  not  only  enhances  our  understanding  of  soft  jammed  materials  but  also  opens  new  avenues  for  applying  fractal  landscape  dynamics  across  different  materials  and  research  fields.
■590    ▼aSchool  code:  0175.
■650  4▼aChemical  engineering
■650  4▼aEnergy
■650  4▼aMaterials  science
■650  4▼aComputational  chemistry
■650  4▼aParticle  physics
■653    ▼aDense  emulsion
■653    ▼aEnergy  landscape
■653    ▼aFractal  landscape  dynamics
■653    ▼aJammed  materials
■653    ▼aRipening  foam
■690    ▼a0542
■690    ▼a0794
■690    ▼a0798
■690    ▼a0219
■690    ▼a0791
■71020▼aUniversity  of  Pennsylvania▼bChemical  and  Biomolecular  Engineering.
■7730  ▼tDissertations  Abstracts  International▼g85-12B.
■790    ▼a0175
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17160675▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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