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Quantitative and Efficient Scanning Transmission Electron Microscopy with Machine Learning
Quantitative and Efficient Scanning Transmission Electron Microscopy with Machine Learning
Quantitative and Efficient Scanning Transmission Electron Microscopy with Machine Learning

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자료유형  
 학위논문 서양
최종처리일시  
20250211153129
ISBN  
9798346874058
DDC  
620.11
저자명  
Wei, Jingrui.
서명/저자  
Quantitative and Efficient Scanning Transmission Electron Microscopy with Machine Learning
발행사항  
[Sl] : The University of Wisconsin - Madison, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
94 p
주기사항  
Source: Dissertations Abstracts International, Volume: 86-06, Section: B.
주기사항  
Advisor: Voyles, Paul M.
학위논문주기  
Thesis (Ph.D.)--The University of Wisconsin - Madison, 2024.
초록/해제  
요약Scanning transmission electron microscopy (STEM) has advanced the field of materials science by enabling atomic-scale structural and functional imaging. Beyond standard 2D imaging, higher dimensional data acquisition and analysis are enabling critical new sample insights. New challenges arise as well from the fast data streaming and big data volume. This thesis will discuss how advanced computational approaches and machine learning (ML) enhance the efficiency of STEM data interpretation with example topics. First, we demonstrate convolutional neural network (CNN) approaches for precise atom localization in high-resolution STEM images, establishing comprehensive benchmarks and investigating the relationship between model characteristics and performance across varying image qualities and content. Second, we introduce a deep learning-based electron counting method for ultrafast 4D-STEM detectors, utilizing a Faster-RCNN architecture to achieve accurate electron event detection at higher electron dose than previous methods. Third, a physics-informed regression model for STEM aberration measurement was developed to provide rapid aberration estimation for fine probe alignment or a starting point for sample phase reconstruction algorithms. Fourth, Z-contrast STEM imaging and 4D-STEM were used to investigate short-range order in high entropy carbides with different compositions and thermal treatment. The thesis concludes with a chapter speculating on future directions for research using ML in electron microscopy. Throughout this work, we highlight the importance of incorporating prior knowledge into the machine learning framework, ranging from data representation to model design, contributing to the broader field of quantitative electron microscopy and automation of STEM analysis.
일반주제명  
Materials science
일반주제명  
Applied physics
일반주제명  
Computational physics
키워드  
Scanning transmission electron microscopy
키워드  
Electron microscopy
키워드  
Machine learning
키워드  
Structure characterization
키워드  
Electron dose
기타저자  
The University of Wisconsin - Madison Materials Science and Engineering
기본자료저록  
Dissertations Abstracts International. 86-06B.
전자적 위치 및 접속  
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■1001  ▼aWei,  Jingrui.
■24510▼aQuantitative  and  Efficient  Scanning  Transmission  Electron  Microscopy  with  Machine  Learning
■260    ▼a[Sl]▼bThe  University  of  Wisconsin  -  Madison▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a94  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  86-06,  Section:  B.
■500    ▼aAdvisor:  Voyles,  Paul  M.
■5021  ▼aThesis  (Ph.D.)--The  University  of  Wisconsin  -  Madison,  2024.
■520    ▼aScanning  transmission  electron  microscopy  (STEM)  has  advanced  the  field  of  materials  science  by  enabling  atomic-scale  structural  and  functional  imaging.  Beyond  standard  2D  imaging,  higher  dimensional  data  acquisition  and  analysis  are  enabling  critical  new  sample  insights.  New  challenges  arise  as  well  from  the  fast  data  streaming  and  big  data  volume.  This  thesis  will  discuss  how  advanced  computational  approaches  and  machine  learning  (ML)  enhance  the  efficiency  of  STEM  data  interpretation  with  example  topics.  First,  we  demonstrate  convolutional  neural  network  (CNN)  approaches  for  precise  atom  localization  in  high-resolution  STEM  images,  establishing  comprehensive  benchmarks  and  investigating  the  relationship  between  model  characteristics  and  performance  across  varying  image  qualities  and  content.  Second,  we  introduce  a  deep  learning-based  electron  counting  method  for  ultrafast  4D-STEM  detectors,  utilizing  a  Faster-RCNN  architecture  to  achieve  accurate  electron  event  detection  at  higher  electron  dose  than  previous  methods.  Third,  a  physics-informed  regression  model  for  STEM  aberration  measurement  was  developed  to  provide  rapid  aberration  estimation  for  fine  probe  alignment  or  a  starting  point  for  sample  phase  reconstruction  algorithms.  Fourth,  Z-contrast  STEM  imaging  and  4D-STEM  were  used  to  investigate  short-range  order  in  high  entropy  carbides  with  different  compositions  and  thermal  treatment.  The  thesis  concludes  with  a  chapter  speculating  on  future  directions  for  research  using  ML  in  electron  microscopy.  Throughout  this  work,  we  highlight  the  importance  of  incorporating  prior  knowledge  into  the  machine  learning  framework,  ranging  from  data  representation  to  model  design,  contributing  to  the  broader  field  of  quantitative  electron  microscopy  and  automation  of  STEM  analysis.
■590    ▼aSchool  code:  0262.
■650  4▼aMaterials  science
■650  4▼aApplied  physics
■650  4▼aComputational  physics
■653    ▼aScanning  transmission  electron  microscopy
■653    ▼aElectron  microscopy
■653    ▼aMachine  learning
■653    ▼aStructure  characterization
■653    ▼aElectron  dose  
■690    ▼a0794
■690    ▼a0800
■690    ▼a0215
■690    ▼a0216
■71020▼aThe  University  of  Wisconsin  -  Madison▼bMaterials  Science  and  Engineering.
■7730  ▼tDissertations  Abstracts  International▼g86-06B.
■790    ▼a0262
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17165150▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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