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Thermalization and Transport in Hyperpolarized Nuclear Spins
Thermalization and Transport in Hyperpolarized Nuclear Spins
Thermalization and Transport in Hyperpolarized Nuclear Spins

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자료유형  
 학위논문 서양
최종처리일시  
20250211151446
ISBN  
9798384452119
DDC  
541
저자명  
Beatrez, William Smith.
서명/저자  
Thermalization and Transport in Hyperpolarized Nuclear Spins
발행사항  
[Sl] : University of California, Berkeley, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
162 p
주기사항  
Source: Dissertations Abstracts International, Volume: 86-03, Section: B.
주기사항  
Advisor: Ajoy, Ashok.
학위논문주기  
Thesis (Ph.D.)--University of California, Berkeley, 2024.
초록/해제  
요약Conventional phases of matter are described in the limit of thermal equilibrium. Recent advances have suggested that periodically driven, non-equilibrium systems can exhibit novel phases of matter with properties that are highly unusual or not possible in their static counterparts. A broad effort is underway to quantify these systems and explore their applications in quantum information science and materials physics. Hyperpolarized nuclear spin systems have properties that are favorable toward enabling these studies. Conventionally probed by Nuclear Magnetic Resonance (NMR), nuclear spins are highly coherent quantum objects that can be controlled via resonant radiofrequency (RF) pulses. This thesis focuses on 13C nuclear spins in diamond, which can be hyperpolarized to highly non-thermal spin state populations via interaction with optically pumped Nitrogen Vacancy (NV) defect centers in the lattice. This hyperpolarization provides a vast acceleration in experiment throughput by ∼ 1010 over conventional thermal NMR, enabling highly precise studies of Floquet prethermalization and discrete time crystalline behavior. Further, two novel techniques for nanoscale magnetic resonance imaging are developed with proofs-of-concept shown using hyperpolarized 13C.
일반주제명  
Physical chemistry
일반주제명  
Quantum physics
일반주제명  
Chemistry
키워드  
Discrete time crystal
키워드  
Floquet prethermalization
키워드  
Hyperpolarization
키워드  
Nitrogen Vacancy
키워드  
Spin diffusion
기타저자  
University of California, Berkeley Chemistry
기본자료저록  
Dissertations Abstracts International. 86-03B.
전자적 위치 및 접속  
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MARC

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■020    ▼a9798384452119
■035    ▼a(MiAaPQ)AAI31296464
■040    ▼aMiAaPQ▼cMiAaPQ
■0820  ▼a541
■1001  ▼aBeatrez,  William  Smith.
■24510▼aThermalization  and  Transport  in  Hyperpolarized  Nuclear  Spins
■260    ▼a[Sl]▼bUniversity  of  California,  Berkeley▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a162  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  86-03,  Section:  B.
■500    ▼aAdvisor:  Ajoy,  Ashok.
■5021  ▼aThesis  (Ph.D.)--University  of  California,  Berkeley,  2024.
■520    ▼aConventional  phases  of  matter  are  described  in  the  limit  of  thermal  equilibrium.  Recent  advances  have  suggested  that  periodically  driven,  non-equilibrium  systems  can  exhibit  novel  phases  of  matter  with  properties  that  are  highly  unusual  or  not  possible  in  their  static  counterparts.  A  broad  effort  is  underway  to  quantify  these  systems  and  explore  their  applications  in  quantum  information  science  and  materials  physics.  Hyperpolarized  nuclear  spin  systems  have  properties  that  are  favorable  toward  enabling  these  studies.  Conventionally  probed  by  Nuclear  Magnetic  Resonance  (NMR),  nuclear  spins  are  highly  coherent  quantum  objects  that  can  be  controlled  via  resonant  radiofrequency  (RF)  pulses.  This  thesis  focuses  on  13C  nuclear  spins  in  diamond,  which  can  be  hyperpolarized  to  highly  non-thermal  spin  state  populations  via  interaction  with  optically  pumped  Nitrogen  Vacancy  (NV)  defect  centers  in  the  lattice.  This  hyperpolarization  provides  a  vast  acceleration  in  experiment  throughput  by  ∼  1010  over  conventional  thermal  NMR,  enabling  highly  precise  studies  of  Floquet  prethermalization  and  discrete  time  crystalline  behavior.  Further,  two  novel  techniques  for  nanoscale  magnetic  resonance  imaging  are  developed  with  proofs-of-concept  shown  using  hyperpolarized  13C.
■590    ▼aSchool  code:  0028.
■650  4▼aPhysical  chemistry
■650  4▼aQuantum  physics
■650  4▼aChemistry
■653    ▼aDiscrete  time  crystal
■653    ▼aFloquet  prethermalization
■653    ▼aHyperpolarization
■653    ▼aNitrogen  Vacancy
■653    ▼aSpin  diffusion
■690    ▼a0494
■690    ▼a0599
■690    ▼a0485
■71020▼aUniversity  of  California,  Berkeley▼bChemistry.
■7730  ▼tDissertations  Abstracts  International▼g86-03B.
■790    ▼a0028
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17161796▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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