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Measuring Spin-Energy Correlations in Nuclear Fission
Measuring Spin-Energy Correlations in Nuclear Fission
Measuring Spin-Energy Correlations in Nuclear Fission

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자료유형  
 학위논문 서양
최종처리일시  
20250211153010
ISBN  
9798384044642
DDC  
539.7
저자명  
Giha, Nathan P.
서명/저자  
Measuring Spin-Energy Correlations in Nuclear Fission
발행사항  
[Sl] : University of Michigan, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
126 p
주기사항  
Source: Dissertations Abstracts International, Volume: 86-03, Section: B.
주기사항  
Advisor: Pozzi, Sara A.;Tovesson, Fredrik.
학위논문주기  
Thesis (Ph.D.)--University of Michigan, 2024.
초록/해제  
요약Despite over eighty years of study since nuclear fission was discovered, important details of this nuclear process remain poorly understood. Among them is the mechanism by which fission fragments acquire substantial spins, or angular momenta, despite originating from a heavy nucleus that may start with no spin. Thanks to advances in computational models of fission, theorists and experimentalists have recently put forth renewed effort toward revealing this spin generation mechanism. A truly predictive model of fission-with the correct spin generation mechanism-would have far-reaching implications on our understanding of fission recycling in the r-process of nucleosynthesis and our ability to simulate fission neutron and γ-ray emission for nuclear safeguards and nonproliferation scenarios.This dissertation aims to measure correlations between the spin generated in the fission fragments and the energy available to them. Practically, we measure correlations between fission γ-ray emission and properties of the fragments that emit them. We first measure the γ-ray multiplicity and spectrum from 239Pu(n,f) as a function of incident neutron energy using the Chi-Nu liquid scintillator array at the Los Alamos Neutron Science Center. We then develop and characterize a specialized fission fragment detector that measures the fragments' kinetic energies and masses at Argonne National Laboratory. Loaded with a 252Cf(sf) source, We place that fragment detector inside Gammasphere, a high-resolution and high-granularity γ-ray spectrometer, to measure correlations between the kinetic energies of specific fragments and γ-ray spectra they emit. We leverage our knowledge of the fragments' nuclear level schemes to reconstruct their spin distributions as a function of energy for the first time. Focusing on 144Ba, we find its average spin to be insensitive to energy-inconsistent with predictions from solely statistical excitation of rotational modes in the fragments. We thus conclude that more complex modes of spin generation are at play in fission.We discuss the corpus of correlated fission measurements that are relevant to spin generation and show how our measurements fit into that collection. We suggest improvements to the presented experiments in case they are repeated in the future, as well as straightforward extensions to the analysis presented in the dissertation with the existing data sets. Finally, we propose future experiments and analyses that will unlock entirely new fragment initial conditions and measured quantities, respectively.
일반주제명  
Nuclear physics
일반주제명  
Nuclear engineering
일반주제명  
Physics
키워드  
Nuclear fission
키워드  
Angular momentum
키워드  
Spin-energy correlations
키워드  
Kinetic energies
키워드  
Spectrometer
기타저자  
University of Michigan Nuclear Engineering & Radiological Sciences
기본자료저록  
Dissertations Abstracts International. 86-03B.
전자적 위치 및 접속  
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MARC

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■1001  ▼aGiha,  Nathan  P.
■24510▼aMeasuring  Spin-Energy  Correlations  in  Nuclear  Fission
■260    ▼a[Sl]▼bUniversity  of  Michigan▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a126  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  86-03,  Section:  B.
■500    ▼aAdvisor:  Pozzi,  Sara  A.;Tovesson,  Fredrik.
■5021  ▼aThesis  (Ph.D.)--University  of  Michigan,  2024.
■520    ▼aDespite  over  eighty  years  of  study  since  nuclear  fission  was  discovered,  important  details  of  this  nuclear  process  remain  poorly  understood.  Among  them  is  the  mechanism  by  which  fission  fragments  acquire  substantial  spins,  or  angular  momenta,  despite  originating  from  a  heavy  nucleus  that  may  start  with  no  spin.  Thanks  to  advances  in  computational  models  of  fission,  theorists  and  experimentalists  have  recently  put  forth  renewed  effort  toward  revealing  this  spin  generation  mechanism.  A  truly  predictive  model  of  fission-with  the  correct  spin  generation  mechanism-would  have  far-reaching  implications  on  our  understanding  of  fission  recycling  in  the  r-process  of  nucleosynthesis  and  our  ability  to  simulate  fission  neutron  and  γ-ray  emission  for  nuclear  safeguards  and  nonproliferation  scenarios.This  dissertation  aims  to  measure  correlations  between  the  spin  generated  in  the  fission  fragments  and  the  energy  available  to  them.  Practically,  we  measure  correlations  between  fission  γ-ray  emission  and  properties  of  the  fragments  that  emit  them.  We  first  measure  the  γ-ray  multiplicity  and  spectrum  from  239Pu(n,f)  as  a  function  of  incident  neutron  energy  using  the  Chi-Nu  liquid  scintillator  array  at  the  Los  Alamos  Neutron  Science  Center.  We  then  develop  and  characterize  a  specialized  fission  fragment  detector  that  measures  the  fragments'  kinetic  energies  and  masses  at  Argonne  National  Laboratory.  Loaded  with  a  252Cf(sf)  source,  We  place  that  fragment  detector  inside  Gammasphere,  a  high-resolution  and  high-granularity  γ-ray  spectrometer,  to  measure  correlations  between  the  kinetic  energies  of  specific  fragments  and  γ-ray  spectra  they  emit.  We  leverage  our  knowledge  of  the  fragments'  nuclear  level  schemes  to  reconstruct  their  spin  distributions  as  a  function  of  energy  for  the  first  time.  Focusing  on  144Ba,  we  find  its  average  spin  to  be  insensitive  to  energy-inconsistent  with  predictions  from  solely  statistical  excitation  of  rotational  modes  in  the  fragments.  We  thus  conclude  that  more  complex  modes  of  spin  generation  are  at  play  in  fission.We  discuss  the  corpus  of  correlated  fission  measurements  that  are  relevant  to  spin  generation  and  show  how  our  measurements  fit  into  that  collection.  We  suggest  improvements  to  the  presented  experiments  in  case  they  are  repeated  in  the  future,  as  well  as  straightforward  extensions  to  the  analysis  presented  in  the  dissertation  with  the  existing  data  sets.  Finally,  we  propose  future  experiments  and  analyses  that  will  unlock  entirely  new  fragment  initial  conditions  and  measured  quantities,  respectively.
■590    ▼aSchool  code:  0127.
■650  4▼aNuclear  physics
■650  4▼aNuclear  engineering
■650  4▼aPhysics
■653    ▼aNuclear  fission
■653    ▼aAngular  momentum
■653    ▼aSpin-energy  correlations
■653    ▼aKinetic  energies
■653    ▼aSpectrometer
■690    ▼a0756
■690    ▼a0552
■690    ▼a0605
■71020▼aUniversity  of  Michigan▼bNuclear  Engineering  &  Radiological  Sciences.
■7730  ▼tDissertations  Abstracts  International▼g86-03B.
■790    ▼a0127
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17164499▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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