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Exploring Topology in Epitaxial Thin Films of Topological Magnets
Exploring Topology in Epitaxial Thin Films of Topological Magnets
Exploring Topology in Epitaxial Thin Films of Topological Magnets

상세정보

자료유형  
 학위논문 서양
최종처리일시  
20250211153107
ISBN  
9798384088950
DDC  
530
저자명  
Cheng, Shuyu.
서명/저자  
Exploring Topology in Epitaxial Thin Films of Topological Magnets
발행사항  
[Sl] : The Ohio State University, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
268 p
주기사항  
Source: Dissertations Abstracts International, Volume: 86-04, Section: B.
주기사항  
Advisor: Kawakami, Roland.
학위논문주기  
Thesis (Ph.D.)--The Ohio State University, 2024.
초록/해제  
요약The concept of "topology" provides a new merit for categorizing materials based on the properties that are not changed under continuous transforms. The introduction of this concept into condensed matter physics has led to the prediction and realization of many exotic quantum states in both momentum space and real space. In momentum space, two topologically distinct insulating states are expected to have a well-defined boundary where a metallic state emerges. In terms of material selection, the kagome lattice inherently manifests Dirac cones and flat bands, which becomes topologically nontrivial in the presence of spin-orbit coupling. In real space, the concept of topology can be used to classify different distributions of order parameters, and the ones with nonzero winding numbers are expected to be more stable since they are topologically protected. The magnetic skyrmions, as prototypical spin textures with a winding number of ?1, are of particular interest for next-generation memory and logic devices.This thesis aims to demonstrate that the nontrivial topology can be realized in thin films via epitaxial growth, where molecular beam epitaxy (MBE) plays a crucial role in controlling the sample structure at the atomic scale. Using MBE, we have synthesized thin films of kagome materials with different magnetic orderings: ferromagnetic Fe3Sn2 (Chapter 3), paramagnetic CoSn (Chapter 4). and ferrimagnetic RMn6Sn6 (Chapter 5), and the magnetic properties of these materials are studied using a combination of the magneto-optical Kerr effect (MOKE) and the superconducting quantum interference device (SQUID) magnetometer. In CoSn, we have directly observed topologically non-trivial flat bands using synchrotron-based angle-resolved photoemission spectroscopy (ARPES). We have also established a quantitative connection between the band structures and the transport properties of CoSn by a semiclassical transport theory. In Chapter 6, we show that the real-space topology can also be manipulated via thin film synthesis. The magnetic properties of [Pt/Co/Cu]N multilayers can be vastly tuned by varying the sample structures, and magnetic skyrmions are observed in those samples with zero-field multidomain states. Finally, in Chapter 7, we will discuss the time- and angle-resolved photoemission spectroscopy at the National Extreme Ultrafast Science (NeXUS) facility, which will become a formidable machine for investigating and manipulating the band topology.
일반주제명  
Physics
일반주제명  
Condensed matter physics
일반주제명  
Physical chemistry
일반주제명  
Materials science
키워드  
Topological materials
키워드  
Magnetic skyrmions
키워드  
Molecular beam epitaxy
키워드  
Angle-resolved photoemission spectroscopy
키워드  
Band topology
기타저자  
The Ohio State University Physics
기본자료저록  
Dissertations Abstracts International. 86-04B.
전자적 위치 및 접속  
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MARC

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■1001  ▼aCheng,  Shuyu.
■24510▼aExploring  Topology  in  Epitaxial  Thin  Films  of  Topological  Magnets
■260    ▼a[Sl]▼bThe  Ohio  State  University▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a268  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  86-04,  Section:  B.
■500    ▼aAdvisor:  Kawakami,  Roland.
■5021  ▼aThesis  (Ph.D.)--The  Ohio  State  University,  2024.
■520    ▼aThe  concept  of  "topology"  provides  a  new  merit  for  categorizing  materials  based  on  the  properties  that  are  not  changed  under  continuous  transforms.  The  introduction  of  this  concept  into  condensed  matter  physics  has  led  to  the  prediction  and  realization  of  many  exotic  quantum  states  in  both  momentum  space  and  real  space.  In  momentum  space,  two  topologically  distinct  insulating  states  are  expected  to  have  a  well-defined  boundary  where  a  metallic  state  emerges.  In  terms  of  material  selection,  the  kagome  lattice  inherently  manifests  Dirac  cones  and  flat  bands,  which  becomes  topologically  nontrivial  in  the  presence  of  spin-orbit  coupling.  In  real  space,  the  concept  of  topology  can  be  used  to  classify  different  distributions  of  order  parameters,  and  the  ones  with  nonzero  winding  numbers  are  expected  to  be  more  stable  since  they  are  topologically  protected.  The  magnetic  skyrmions,  as  prototypical  spin  textures  with  a  winding  number  of  ?1,  are  of  particular  interest  for  next-generation  memory  and  logic  devices.This  thesis  aims  to  demonstrate  that  the  nontrivial  topology  can  be  realized  in  thin  films  via  epitaxial  growth,  where  molecular  beam  epitaxy  (MBE)  plays  a  crucial  role  in  controlling  the  sample  structure  at  the  atomic  scale.  Using  MBE,  we  have  synthesized  thin  films  of  kagome  materials  with  different  magnetic  orderings:  ferromagnetic  Fe3Sn2  (Chapter  3),  paramagnetic  CoSn  (Chapter  4).  and  ferrimagnetic  RMn6Sn6  (Chapter  5),  and  the  magnetic  properties  of  these  materials  are  studied  using  a  combination  of  the  magneto-optical  Kerr  effect  (MOKE)  and  the  superconducting  quantum  interference  device  (SQUID)  magnetometer.  In  CoSn,  we  have  directly  observed  topologically  non-trivial  flat  bands  using  synchrotron-based  angle-resolved  photoemission  spectroscopy  (ARPES).  We  have  also  established  a  quantitative  connection  between  the  band  structures  and  the  transport  properties  of  CoSn  by  a  semiclassical  transport  theory.  In  Chapter  6,  we  show  that  the  real-space  topology  can  also  be  manipulated  via  thin  film  synthesis.  The  magnetic  properties  of  [Pt/Co/Cu]N  multilayers  can  be  vastly  tuned  by  varying  the  sample  structures,  and  magnetic  skyrmions  are  observed  in  those  samples  with  zero-field  multidomain  states.  Finally,  in  Chapter  7,  we  will  discuss  the  time-  and  angle-resolved  photoemission  spectroscopy  at  the  National  Extreme  Ultrafast  Science  (NeXUS)  facility,  which  will  become  a  formidable  machine  for  investigating  and  manipulating  the  band  topology.
■590    ▼aSchool  code:  0168.
■650  4▼aPhysics
■650  4▼aCondensed  matter  physics
■650  4▼aPhysical  chemistry
■650  4▼aMaterials  science
■653    ▼aTopological  materials
■653    ▼aMagnetic  skyrmions
■653    ▼aMolecular  beam  epitaxy
■653    ▼aAngle-resolved  photoemission  spectroscopy
■653    ▼aBand  topology
■690    ▼a0611
■690    ▼a0605
■690    ▼a0794
■690    ▼a0494
■71020▼aThe  Ohio  State  University▼bPhysics.
■7730  ▼tDissertations  Abstracts  International▼g86-04B.
■790    ▼a0168
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17164954▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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