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Characterization of a 4He Scintillation Detector and Its Applications in Nuclear Material Assay
Characterization of a 4He Scintillation Detector and Its Applications in Nuclear Material ...
Characterization of a 4He Scintillation Detector and Its Applications in Nuclear Material Assay

상세정보

자료유형  
 학위논문 서양
최종처리일시  
20250211152106
ISBN  
9798382741109
DDC  
539.7
저자명  
Searfus, Oskar Fick.
서명/저자  
Characterization of a 4He Scintillation Detector and Its Applications in Nuclear Material Assay
발행사항  
[Sl] : University of Michigan, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
154 p
주기사항  
Source: Dissertations Abstracts International, Volume: 85-12, Section: B.
주기사항  
Advisor: Jovanovic, Igor.
학위논문주기  
Thesis (Ph.D.)--University of Michigan, 2024.
초록/해제  
요약Helium-4-based scintillation detectors have been developed as a gamma-insensitive alternative to organic scintillators for fast neutron detection and spectroscopy. While these detectors hold significant promise for applications in extreme environments where organic scintillators are not suitable, there has been relatively little scholarship on their fundamental characteristics and applications. The only commercially available He-4-based detector is the Arktis S670. This detector has a unique construction, containing three optically segmented regions, each providing four signal outputs. An algorithm was developed to condense these four outputs into a single data list, showing an improved time resolution compared to a separate analysis of the outputs, and an energy calibration using monoenergetic 2.45 MeV and 14.1 MeV neutrons was demonstrated. Another experiment was performed to characterize the response of the He-4 detector to monoenergetic nuclear recoils up to 9 MeV. The He-4 detector was positioned in the center of a semicircular array of organic scintillation detectors operated in coincidence, in conjunction with monoenergetic neutron sources. The measured detector response provides evidence for scintillation linearity and was used to develop an energy resolution function applicable to this energy range, enabling high-fidelity detector simulation for future applications. Precise knowledge of the temporal output profile of a pulsed neutron generator is beneficial for several neutron active interrogation techniques. Using the He-4 detector, the primary temporal profile of a short-pulsed deuterium-tritium neutron generator was isolated from scattered and induced contaminants by spectral thresholding. This method can be used to continuously monitor the pulse characteristics and quality for various neutron active interrogation techniques. The production of U-233 poses unique challenges for nuclear safeguards, as it is associated with an extreme gamma ray environment from U-232 contamination, as well as more conservative accountability requirements than for U-235. The He-4 detector and an array of He-3 detectors were used to demonstrate three advanced neutron signatures of U-233 in oxide. These measurements provide a benchmark for future nondestructive assay instrumentation development and demonstrate a set of key neutron signatures to be leveraged for nuclear safeguards in the thorium fuel cycle. The use of photon active interrogation for the detection of special nuclear material has held significant promise; however, neutrons produced by photonuclear reactions in the accelerator target, collimator, and environment can obscure the fission neutron signal. High-pressure He-4-based scintillation detectors are well-suited to photon active interrogation, as they can measure the fast neutron spectrum, but show little response to gamma rays. A photon active interrogation system utilizing a He-4 scintillation detector and a 9 MeV linac-bremsstrahlung X-ray source was experimentally evaluated. It was shown to be capable of detecting photofission neutrons from U-238 based on their clear spectral separation from (gamma,n) neutrons produced in lead, a common shielding material. This collection of research serves to deepen the understanding of He-4-based detector characteristics and pioneer some of their promising applications in nuclear safeguards and security. While additional work remains to develop the demonstrated applications into operational systems, this work has significantly broadened the plausible application space for He-4 scintillation detectors.
일반주제명  
Nuclear physics
일반주제명  
Nuclear engineering
일반주제명  
Nuclear chemistry
키워드  
Fast neutrons
키워드  
Neutron detection
키워드  
Nuclear security
키워드  
Nuclear safeguards
키워드  
He-4
기타저자  
University of Michigan Nuclear Engineering & Radiological Sciences
기본자료저록  
Dissertations Abstracts International. 85-12B.
전자적 위치 및 접속  
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MARC

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■020    ▼a9798382741109
■035    ▼a(MiAaPQ)AAI31349098
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■0820  ▼a539.7
■1001  ▼aSearfus,  Oskar  Fick.
■24510▼aCharacterization  of  a  4He  Scintillation  Detector  and  Its  Applications  in  Nuclear  Material  Assay
■260    ▼a[Sl]▼bUniversity  of  Michigan▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a154  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  85-12,  Section:  B.
■500    ▼aAdvisor:  Jovanovic,  Igor.
■5021  ▼aThesis  (Ph.D.)--University  of  Michigan,  2024.
■520    ▼aHelium-4-based  scintillation  detectors  have  been  developed  as  a  gamma-insensitive  alternative  to  organic  scintillators  for  fast  neutron  detection  and  spectroscopy.  While  these  detectors  hold  significant  promise  for  applications  in  extreme  environments  where  organic  scintillators  are  not  suitable,  there  has  been  relatively  little  scholarship  on  their  fundamental  characteristics  and  applications.  The  only  commercially  available  He-4-based  detector  is  the  Arktis  S670.  This  detector  has  a  unique  construction,  containing  three  optically  segmented  regions,  each  providing  four  signal  outputs.  An  algorithm  was  developed  to  condense  these  four  outputs  into  a  single  data  list,  showing  an  improved  time  resolution  compared  to  a  separate  analysis  of  the  outputs,  and  an  energy  calibration  using  monoenergetic  2.45  MeV  and  14.1  MeV  neutrons  was  demonstrated.  Another  experiment  was  performed  to  characterize  the  response  of  the  He-4  detector  to  monoenergetic  nuclear  recoils  up  to  9  MeV.  The  He-4  detector  was  positioned  in  the  center  of  a  semicircular  array  of  organic  scintillation  detectors  operated  in  coincidence,  in  conjunction  with  monoenergetic  neutron  sources.  The  measured  detector  response  provides  evidence  for  scintillation  linearity  and  was  used  to  develop  an  energy  resolution  function  applicable  to  this  energy  range,  enabling  high-fidelity  detector  simulation  for  future  applications.  Precise  knowledge  of  the  temporal  output  profile  of  a  pulsed  neutron  generator  is  beneficial  for  several  neutron  active  interrogation  techniques.  Using  the  He-4  detector,  the  primary  temporal  profile  of  a  short-pulsed  deuterium-tritium  neutron  generator  was  isolated  from  scattered  and  induced  contaminants  by  spectral  thresholding.  This  method  can  be  used  to  continuously  monitor  the  pulse  characteristics  and  quality  for  various  neutron  active  interrogation  techniques.  The  production  of  U-233  poses  unique  challenges  for  nuclear  safeguards,  as  it  is  associated  with  an  extreme  gamma  ray  environment  from  U-232  contamination,  as  well  as  more  conservative  accountability  requirements  than  for  U-235.  The  He-4  detector  and  an  array  of  He-3  detectors  were  used  to  demonstrate  three  advanced  neutron  signatures  of  U-233  in  oxide.  These  measurements  provide  a  benchmark  for  future  nondestructive  assay  instrumentation  development  and  demonstrate  a  set  of  key  neutron  signatures  to  be  leveraged  for  nuclear  safeguards  in  the  thorium  fuel  cycle.  The  use  of  photon  active  interrogation  for  the  detection  of  special  nuclear  material  has  held  significant  promise;  however,  neutrons  produced  by  photonuclear  reactions  in  the  accelerator  target,  collimator,  and  environment  can  obscure  the  fission  neutron  signal.  High-pressure  He-4-based  scintillation  detectors  are  well-suited  to  photon  active  interrogation,  as  they  can  measure  the  fast  neutron  spectrum,  but  show  little  response  to  gamma  rays.  A  photon  active  interrogation  system  utilizing  a  He-4  scintillation  detector  and  a  9  MeV  linac-bremsstrahlung  X-ray  source  was  experimentally  evaluated.  It  was  shown  to  be  capable  of  detecting  photofission  neutrons  from  U-238  based  on  their  clear  spectral  separation  from  (gamma,n)  neutrons  produced  in  lead,  a  common  shielding  material.  This  collection  of  research  serves  to  deepen  the  understanding  of  He-4-based  detector  characteristics  and  pioneer  some  of  their  promising  applications  in  nuclear  safeguards  and  security.  While  additional  work  remains  to  develop  the  demonstrated  applications  into  operational  systems,  this  work  has  significantly  broadened  the  plausible  application  space  for  He-4  scintillation  detectors.
■590    ▼aSchool  code:  0127.
■650  4▼aNuclear  physics
■650  4▼aNuclear  engineering
■650  4▼aNuclear  chemistry
■653    ▼aFast  neutrons
■653    ▼aNeutron  detection
■653    ▼aNuclear  security
■653    ▼aNuclear  safeguards
■653    ▼aHe-4
■690    ▼a0552
■690    ▼a0756
■690    ▼a0738
■71020▼aUniversity  of  Michigan▼bNuclear  Engineering  &  Radiological  Sciences.
■7730  ▼tDissertations  Abstracts  International▼g85-12B.
■790    ▼a0127
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17162869▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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