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Non-contact Measurements of Nanoscale Phonon and Electron Transport with Ultrafast, Coherent Short-Wavelength Light
Non-contact Measurements of Nanoscale Phonon and Electron Transport with Ultrafast, Cohere...
Non-contact Measurements of Nanoscale Phonon and Electron Transport with Ultrafast, Coherent Short-Wavelength Light

Detailed Information

자료유형  
 학위논문 서양
최종처리일시  
20250211152038
ISBN  
9798384052272
DDC  
530
저자명  
McBennett, Brendan Gray.
서명/저자  
Non-contact Measurements of Nanoscale Phonon and Electron Transport with Ultrafast, Coherent Short-Wavelength Light
발행사항  
[Sl] : University of Colorado at Boulder, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
197 p
주기사항  
Source: Dissertations Abstracts International, Volume: 86-03, Section: B.
주기사항  
Advisor: Murnane, Margaret.
학위논문주기  
Thesis (Ph.D.)--University of Colorado at Boulder, 2024.
초록/해제  
요약The miniaturization of technology over the past few decades has generated enormous demand for experimental techniques capable of resolving material dynamics at ever shorter length and time scales. Ultrafast, coherent ultraviolet light provides a window into microscopic dynamics, combining femtosecond pulse durations, short wavelengths and tunable sensitivity to electronic and thermal processes. This thesis furthers the development of novel ultraviolet metrology tools and their application to nanoscale phonon and electron transport, where confinement and nonequilibrium conditions give rise to surprising new phenomena. Using extreme ultraviolet scatterometry, we extract the thermal and elastic properties of a 3D phononic crystal metalattice, nanostructured on 100 nm length scales, and combine the results with previous experiments and atomistic simulations to propose a new effective description of highly-confined heat flow in nanostructured semiconductors. An interlude discusses the challenges associated with contact- and fabrication-based approaches to studying transport phenomena in the context of the wider array of materials appearing in modern nanotechnology. The final chapter introduces a new non-contact deep-ultraviolet (6.3 eV) transient grating experiment, capable of investigating nanoscale phonon and electron transport in ultrawide-bandgap materials at femtosecond timescales. This new technique bridges previous laboratory and facility-scale capabilities and provides new opportunities for studying emergent nanoscale transport phenomena of relevance to next-generation energy and semiconductor technologies.
일반주제명  
Physics
일반주제명  
Applied physics
일반주제명  
Nanotechnology
일반주제명  
Optics
키워드  
Scatterometry
키워드  
Semiconductor technologies
키워드  
Femtosecond pulse durations
기타저자  
University of Colorado at Boulder Physics
기본자료저록  
Dissertations Abstracts International. 86-03B.
전자적 위치 및 접속  
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MARC

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■1001  ▼aMcBennett,  Brendan  Gray.▼0(orcid)0000-0001-7947-6551
■24510▼aNon-contact  Measurements  of  Nanoscale  Phonon  and  Electron  Transport  with  Ultrafast,  Coherent  Short-Wavelength  Light
■260    ▼a[Sl]▼bUniversity  of  Colorado  at  Boulder▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a197  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  86-03,  Section:  B.
■500    ▼aAdvisor:  Murnane,  Margaret.
■5021  ▼aThesis  (Ph.D.)--University  of  Colorado  at  Boulder,  2024.
■520    ▼aThe  miniaturization  of  technology  over  the  past  few  decades  has  generated  enormous  demand  for  experimental  techniques  capable  of  resolving  material  dynamics  at  ever  shorter  length  and  time  scales.  Ultrafast,  coherent  ultraviolet  light  provides  a  window  into  microscopic  dynamics,  combining  femtosecond  pulse  durations,  short  wavelengths  and  tunable  sensitivity  to  electronic  and  thermal  processes.  This  thesis  furthers  the  development  of  novel  ultraviolet  metrology  tools  and  their  application  to  nanoscale  phonon  and  electron  transport,  where  confinement  and  nonequilibrium  conditions  give  rise  to  surprising  new  phenomena.  Using  extreme  ultraviolet  scatterometry,  we  extract  the  thermal  and  elastic  properties  of  a  3D  phononic  crystal  metalattice,  nanostructured  on  100  nm  length  scales,  and  combine  the  results  with  previous  experiments  and  atomistic  simulations  to  propose  a  new  effective  description  of  highly-confined  heat  flow  in  nanostructured  semiconductors.  An  interlude  discusses  the  challenges  associated  with  contact-  and  fabrication-based  approaches  to  studying  transport  phenomena  in  the  context  of  the  wider  array  of  materials  appearing  in  modern  nanotechnology.  The  final  chapter  introduces  a  new  non-contact  deep-ultraviolet  (6.3  eV)  transient  grating  experiment,  capable  of  investigating  nanoscale  phonon  and  electron  transport  in  ultrawide-bandgap  materials  at  femtosecond  timescales.  This  new  technique  bridges  previous  laboratory  and  facility-scale  capabilities  and  provides  new  opportunities  for  studying  emergent  nanoscale  transport  phenomena  of  relevance  to  next-generation  energy  and  semiconductor  technologies.
■590    ▼aSchool  code:  0051.
■650  4▼aPhysics
■650  4▼aApplied  physics
■650  4▼aNanotechnology
■650  4▼aOptics
■653    ▼aScatterometry
■653    ▼aSemiconductor  technologies
■653    ▼aFemtosecond  pulse  durations
■690    ▼a0605
■690    ▼a0752
■690    ▼a0652
■690    ▼a0215
■71020▼aUniversity  of  Colorado  at  Boulder▼bPhysics.
■7730  ▼tDissertations  Abstracts  International▼g86-03B.
■790    ▼a0051
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17162662▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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