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Characterizing Desorbed Surface Contaminants Leading to Plasma Formation in Power Feeds of Pulsed Power Accelerators
Characterizing Desorbed Surface Contaminants Leading to Plasma Formation in Power Feeds of...
Characterizing Desorbed Surface Contaminants Leading to Plasma Formation in Power Feeds of Pulsed Power Accelerators

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자료유형  
 학위논문 서양
최종처리일시  
20260202105235
ISBN  
9798291567784
DDC  
530
저자명  
Smith, Trevor Johannes.
서명/저자  
Characterizing Desorbed Surface Contaminants Leading to Plasma Formation in Power Feeds of Pulsed Power Accelerators
발행사항  
[Sl] : University of Michigan, 2025
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2025
형태사항  
204 p
주기사항  
Source: Dissertations Abstracts International, Volume: 87-02, Section: B.
주기사항  
Advisor: McBride, Ryan David.
학위논문주기  
Thesis (Ph.D.)--University of Michigan, 2025.
초록/해제  
요약The Z machine at Sandia National Laboratories delivers a 20-30 MA current pulse to various experimental load configurations in as little as 100 ns. The pulse is transported to the load via magnetically insulated transmission lines (MITLs), which are nominally vacuum filled. However, measurements show that plasma forms in the MITLs and that not all the current makes it to the load.It is suspected that under shot ready vacuum conditions ( 3x10−5 Torr), a few monolayers of contaminants, particularly water, are present on the surfaces of the MITL electrodes. This is supported by previous visible spectroscopy measurements in the post-hole convolute and inner MITL regions on Z. As the current pulse ohmically heats the electrode material, the neutral surface contaminants ionize and break down into a plasma that can conduct current across the anode-cathode gap, limiting the total current delivered to the load.The goal of this dissertation research was to develop new techniques to study and characterize low-density power feed plasmas relevant to the Z facility using smaller and more accessible pulsed power drivers, such as the 1-MA, 100-ns MAIZE facility at the University of Michigan and the 1-MA, 100-ns Mykonos facility at Sandia National Laboratories. The hope is that some of the techniques developed (e.g., VUV spectroscopy) can be transferred to the Z facility in the future. A significant challenge to this research, however, is that on 1-MA-scale facilities, the electrode heating rates are typically not sufficient for generating detectable levels of low-density power feed plasma. Thus, the first step in this dissertation research was to develop a new platform for 1-MA drivers that mimics the electrode plasma formation found on the much larger Z facility. The new platform developed consists of a stripline structure that uses thin-foil electrode surfaces (5-500 μm thick) to increase the current densities and local heating rates in 1-MA-scale experiments. The foils are backed by 3D printed dielectric structures to maintain electrode shape during the experiment. By varying the foil thickness, the current density and heating rates are controlled. Using this platform on MAIZE, high-speed imaging revealed gap-closure velocities of 1-10 cm/μs, which is comparable to the gap-closure velocities found on Z.With the platform developed, the aim of this research then shifted to identifying and quantifying the contaminant species that desorb off the thin-foil stripline surfaces during 1-MA discharges. With the ultimate goal being to understand how desorbed neutral contaminants affect the breakdown process, vacuum-ultraviolet (VUV) and visible-light spectroscopy were used to measure the neutral densities and temperatures of contaminant species within the stripline structure before, during, and after breakdown.For this dissertation, the neutral atomic hydrogen density with spatial resolution across the stripline anode-cathode gap was measured. This was done using a gated vacuum ultraviolet spectrometer to collect and analyze the absolute line intensity of the hydrogen Lyman-a transition. The VUV spectra collected prior to breakdown show a Lyman-a transition density of 109-1010 transitions/cm3, indicating an atomic hydrogen number density of 1012-1013 particles/cm3. After breakdown, a Lyman-a transition density of 1011-1012 transitions/cm3, was measured indicating that the neutral hydrogen number density had increased to 1013- 1014 particles/cm3. The ratios between molecular hydrogen bands indicates that the temperature is in the range of 5000-6000 K before breakdown and 5000-9000 K after breakdown.From the post-breakdown VUV measurements, there is a correlation between the decrease in transition densities of the lower order molecular hydrogen Lyman band, an increase in transition densities of the higher order molecular hydrogen Werner band, and an increase in the atomic hydrogen Lyman-α transition densities. This shows shows a distinct change in energetics of the neutrals present, as the pathways for molecular hydrogen dissociation into atomic hydrogen through collisions with electrons occur at higher temperatures. This change in energetics, leading to a change in molecular and atomic populations, can be seen in the population rate coefficients from collisional radiative modeling. Additionally, after breakdown, the VUV data show that atomic and molecular hydrogen is still present in the anode-cathode gap, indicating that not all of the contaminant particles are ionized after breakdown, as previously thought.Streaked visible spectroscopy (SVS) was used to collect graybody spectra from the stripline's cathode surface. This was done by focusing the SVS collection optics onto the cathode surface and using a line of sight with at least a small component normal to the cathode surface. From the graybody data collected after breakdown (i.e., after plasma formation), plasma temperatures in the range of 1-2 eV were inferred.The SVS system was also fielded with a side-on view of the stripline's anode-cathode gap (i.e., with a line of sight that is orthogonal to the plane set by the stripline's gap). This was done to collect line-emission spectra from the plasma that filled the space between the stripline's anode and cathode. The line-emission spectra was used to identify the various species present. For example, early in time, oxygen was found to be present. The oxygen's presence then persisted into late times, when iron became detectable, indicating that the stripline's foil surface had melted, and when gaseous and ionized elements of the foil material had begun to cross the anode-cathode gap.The experimental data presented in this dissertation will be helpful to researchers who are presently developing models of contaminant plasma formation in high-power MITLs.
일반주제명  
Physics
일반주제명  
Electromagnetics
일반주제명  
Plasma physics
일반주제명  
Optics
키워드  
Surface contaminants
키워드  
Plasma formation
키워드  
Pulsed power accelerators
키워드  
Magnetically insulated transmission lines
키워드  
Spectroscopy
기타저자  
University of Michigan Nuclear Engineering & Radiological Sciences
기본자료저록  
Dissertations Abstracts International. 87-02B.
전자적 위치 및 접속  
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MARC

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■1001  ▼aSmith,  Trevor  Johannes.
■24510▼aCharacterizing  Desorbed  Surface  Contaminants  Leading  to  Plasma  Formation  in  Power  Feeds  of  Pulsed  Power  Accelerators
■260    ▼a[Sl]▼bUniversity  of  Michigan▼c2025
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2025
■300    ▼a204  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  87-02,  Section:  B.
■500    ▼aAdvisor:  McBride,  Ryan  David.
■5021  ▼aThesis  (Ph.D.)--University  of  Michigan,  2025.
■520    ▼aThe  Z  machine  at  Sandia  National  Laboratories  delivers  a  20-30  MA  current  pulse  to  various  experimental  load  configurations  in  as  little  as  100  ns.  The  pulse  is  transported  to  the  load  via  magnetically  insulated  transmission  lines  (MITLs),  which  are  nominally  vacuum  filled.  However,  measurements  show  that  plasma  forms  in  the  MITLs  and  that  not  all  the  current  makes  it  to  the  load.It  is  suspected  that  under  shot  ready  vacuum  conditions  (  3x10−5  Torr),  a  few  monolayers  of  contaminants,  particularly  water,  are  present  on  the  surfaces  of  the  MITL  electrodes.  This  is  supported  by  previous  visible  spectroscopy  measurements  in  the  post-hole  convolute  and  inner  MITL  regions  on  Z.  As  the  current  pulse  ohmically  heats  the  electrode  material,  the  neutral  surface  contaminants  ionize  and  break  down  into  a  plasma  that  can  conduct  current  across  the  anode-cathode  gap,  limiting  the  total  current  delivered  to  the  load.The  goal  of  this  dissertation  research  was  to  develop  new  techniques  to  study  and  characterize  low-density  power  feed  plasmas  relevant  to  the  Z  facility  using  smaller  and  more  accessible  pulsed  power  drivers,  such  as  the  1-MA,  100-ns  MAIZE  facility  at  the  University  of  Michigan  and  the  1-MA,  100-ns  Mykonos  facility  at  Sandia  National  Laboratories.  The  hope  is  that  some  of  the  techniques  developed  (e.g.,  VUV  spectroscopy)  can  be  transferred  to  the  Z  facility  in  the  future.  A  significant  challenge  to  this  research,  however,  is  that  on  1-MA-scale  facilities,  the  electrode  heating  rates  are  typically  not  sufficient  for  generating  detectable  levels  of  low-density  power  feed  plasma.  Thus,  the  first  step  in  this  dissertation  research  was  to  develop  a  new  platform  for  1-MA  drivers  that  mimics  the  electrode  plasma  formation  found  on  the  much  larger  Z  facility.  The  new  platform  developed  consists  of  a  stripline  structure  that  uses  thin-foil  electrode  surfaces  (5-500  μm  thick)  to  increase  the  current  densities  and  local  heating  rates  in  1-MA-scale  experiments.  The  foils  are  backed  by  3D  printed  dielectric  structures  to  maintain  electrode  shape  during  the  experiment.  By  varying  the  foil  thickness,  the  current  density  and  heating  rates  are  controlled.  Using  this  platform  on  MAIZE,  high-speed  imaging  revealed  gap-closure  velocities  of  1-10  cm/μs,  which  is  comparable  to  the  gap-closure  velocities  found  on  Z.With  the  platform  developed,  the  aim  of  this  research  then  shifted  to  identifying  and  quantifying  the  contaminant  species  that  desorb  off  the  thin-foil  stripline  surfaces  during  1-MA  discharges.  With  the  ultimate  goal  being  to  understand  how  desorbed  neutral  contaminants  affect  the  breakdown  process,  vacuum-ultraviolet  (VUV)  and  visible-light  spectroscopy  were  used  to  measure  the  neutral  densities  and  temperatures  of  contaminant  species  within  the  stripline  structure  before,  during,  and  after  breakdown.For  this  dissertation,  the  neutral  atomic  hydrogen  density  with  spatial  resolution  across  the  stripline  anode-cathode  gap  was  measured.  This  was  done  using  a  gated  vacuum  ultraviolet  spectrometer  to  collect  and  analyze  the  absolute  line  intensity  of  the  hydrogen  Lyman-a  transition.  The  VUV  spectra  collected  prior  to  breakdown  show  a  Lyman-a  transition  density  of  109-1010  transitions/cm3,  indicating  an  atomic  hydrogen  number  density  of  1012-1013  particles/cm3.  After  breakdown,  a  Lyman-a  transition  density  of  1011-1012  transitions/cm3,  was  measured  indicating  that  the  neutral  hydrogen  number  density  had  increased  to  1013-  1014  particles/cm3.  The  ratios  between  molecular  hydrogen  bands  indicates  that  the  temperature  is  in  the  range  of  5000-6000  K  before  breakdown  and  5000-9000  K  after  breakdown.From  the  post-breakdown  VUV  measurements,  there  is  a  correlation  between  the  decrease  in  transition  densities  of  the  lower  order  molecular  hydrogen  Lyman  band,  an  increase  in  transition  densities  of  the  higher  order  molecular  hydrogen  Werner  band,  and  an  increase  in  the  atomic  hydrogen  Lyman-α  transition  densities.  This  shows  shows  a  distinct  change  in  energetics  of  the  neutrals  present,  as  the  pathways  for  molecular  hydrogen  dissociation  into  atomic  hydrogen  through  collisions  with  electrons  occur  at  higher  temperatures.  This  change  in  energetics,  leading  to  a  change  in  molecular  and  atomic  populations,  can  be  seen  in  the  population  rate  coefficients  from  collisional  radiative  modeling.  Additionally,  after  breakdown,  the  VUV  data  show  that  atomic  and  molecular  hydrogen  is  still  present  in  the  anode-cathode  gap,  indicating  that  not  all  of  the  contaminant  particles  are  ionized  after  breakdown,  as  previously  thought.Streaked  visible  spectroscopy  (SVS)  was  used  to  collect  graybody  spectra  from  the  stripline's  cathode  surface.  This  was  done  by  focusing  the  SVS  collection  optics  onto  the  cathode  surface  and  using  a  line  of  sight  with  at  least  a  small  component  normal  to  the  cathode  surface.  From  the  graybody  data  collected  after  breakdown  (i.e.,  after  plasma  formation),  plasma  temperatures  in  the  range  of  1-2  eV  were  inferred.The  SVS  system  was  also  fielded  with  a  side-on  view  of  the  stripline's  anode-cathode  gap  (i.e.,  with  a  line  of  sight  that  is  orthogonal  to  the  plane  set  by  the  stripline's  gap).  This  was  done  to  collect  line-emission  spectra  from  the  plasma  that  filled  the  space  between  the  stripline's  anode  and  cathode.  The  line-emission  spectra  was  used  to  identify  the  various  species  present.  For  example,  early  in  time,  oxygen  was  found  to  be  present.  The  oxygen's  presence  then  persisted  into  late  times,  when  iron  became  detectable,  indicating  that  the  stripline's  foil  surface  had  melted,  and  when  gaseous  and  ionized  elements  of  the  foil  material  had  begun  to  cross  the  anode-cathode  gap.The  experimental  data  presented  in  this  dissertation  will  be  helpful  to  researchers  who  are  presently  developing  models  of  contaminant  plasma  formation  in  high-power  MITLs.
■590    ▼aSchool  code:  0127.
■650  4▼aPhysics
■650  4▼aElectromagnetics
■650  4▼aPlasma  physics
■650  4▼aOptics
■653    ▼aSurface  contaminants
■653    ▼aPlasma  formation
■653    ▼aPulsed  power  accelerators
■653    ▼aMagnetically  insulated  transmission  lines
■653    ▼aSpectroscopy
■690    ▼a0605
■690    ▼a0752
■690    ▼a0607
■690    ▼a0759
■71020▼aUniversity  of  Michigan▼bNuclear  Engineering  &  Radiological  Sciences.
■7730  ▼tDissertations  Abstracts  International▼g87-02B.
■790    ▼a0127
■791    ▼aPh.D.
■792    ▼a2025
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17359916▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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