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Soft Chemical Methods to Achieve Novel Quantum Materials
Soft Chemical Methods to Achieve Novel Quantum Materials
Soft Chemical Methods to Achieve Novel Quantum Materials

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자료유형  
 학위논문 서양
최종처리일시  
20260202103516
ISBN  
9798280747241
DDC  
540
저자명  
Hoff, Brianna L.
서명/저자  
Soft Chemical Methods to Achieve Novel Quantum Materials
발행사항  
[Sl] : Princeton University, 2025
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2025
형태사항  
145 p
주기사항  
Source: Dissertations Abstracts International, Volume: 86-12, Section: B.
주기사항  
Advisor: Schoop, Leslie M.
학위논문주기  
Thesis (Ph.D.)--Princeton University, 2025.
초록/해제  
요약As technology continues to grow, so too does the need for new materials. However, we are reaching the limits of conventional materials, necessitating the study of new types of materials with properties that exhibit non-classical physics, known as quantum materials. This dissertation explores the various ways in which soft-chemical methods are used to obtain two types of quantum materials: low-dimensional and superconducting. We find that chemical exfoliation provides access to nanosheets of the non-layered material, Bi2O3, as well as CrSe2 nanoribbons, and CrTe2-x nanosheets. Together, these three systems showcase the versatility of chemical exfoliation in terms of material class, structure type, and morphology. We also demonstrate soft-chemical methods for preparing superconducting 2M-WS2 and show how gentler methods can achieve higher-quality crystals. We support this claim through magnetic susceptibility and heat capacity measurements in a comparison study between 2M-WS2 prepared with soft and aggressive reagents. We also report the synthesis of two new layered materials, NaW2S4 and RbxWS2, and show how both materials can be used for the preparation of high-quality 2M-WS2.
일반주제명  
Chemistry
일반주제명  
Materials science
일반주제명  
Condensed matter physics
일반주제명  
Physical chemistry
일반주제명  
Nanotechnology
키워드  
Chemical exfoliation
키워드  
Low-dimensional
키워드  
Nanomaterials
키워드  
Quantum materials
키워드  
Superconductivity
키워드  
Two-dimensional materials
기타저자  
Princeton University Chemistry
기본자료저록  
Dissertations Abstracts International. 86-12B.
전자적 위치 및 접속  
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MARC

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■035    ▼a(MiAaPQ)AAI32038256
■040    ▼aMiAaPQ▼cMiAaPQ
■0820  ▼a540
■1001  ▼aHoff,  Brianna  L.▼0(orcid)0000-0002-1971-8931
■24510▼aSoft  Chemical  Methods  to  Achieve  Novel  Quantum  Materials
■260    ▼a[Sl]▼bPrinceton  University▼c2025
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2025
■300    ▼a145  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  86-12,  Section:  B.
■500    ▼aAdvisor:  Schoop,  Leslie  M.
■5021  ▼aThesis  (Ph.D.)--Princeton  University,  2025.
■520    ▼aAs  technology  continues  to  grow,  so  too  does  the  need  for  new  materials.  However,  we  are  reaching  the  limits  of  conventional  materials,  necessitating  the  study  of  new  types  of  materials  with  properties  that  exhibit  non-classical  physics,  known  as  quantum  materials.  This  dissertation  explores  the  various  ways  in  which  soft-chemical  methods  are  used  to  obtain  two  types  of  quantum  materials:  low-dimensional  and  superconducting.  We  find  that  chemical  exfoliation  provides  access  to  nanosheets  of  the  non-layered  material,  Bi2O3,  as  well  as  CrSe2  nanoribbons,  and  CrTe2-x  nanosheets.  Together,  these  three  systems  showcase  the  versatility  of  chemical  exfoliation  in  terms  of  material  class,  structure  type,  and  morphology.  We  also  demonstrate  soft-chemical  methods  for  preparing  superconducting  2M-WS2  and  show  how  gentler  methods  can  achieve  higher-quality  crystals.  We  support  this  claim  through  magnetic  susceptibility  and  heat  capacity  measurements  in  a  comparison  study  between  2M-WS2  prepared  with  soft  and  aggressive  reagents.  We  also  report  the  synthesis  of  two  new  layered  materials,  NaW2S4  and  RbxWS2,  and  show  how  both  materials  can  be  used  for  the  preparation  of  high-quality  2M-WS2.
■590    ▼aSchool  code:  0181.
■650  4▼aChemistry
■650  4▼aMaterials  science
■650  4▼aCondensed  matter  physics
■650  4▼aPhysical  chemistry
■650  4▼aNanotechnology
■653    ▼aChemical  exfoliation
■653    ▼aLow-dimensional
■653    ▼aNanomaterials
■653    ▼aQuantum  materials
■653    ▼aSuperconductivity
■653    ▼aTwo-dimensional  materials
■690    ▼a0485
■690    ▼a0794
■690    ▼a0652
■690    ▼a0611
■690    ▼a0494
■71020▼aPrinceton  University▼bChemistry.
■7730  ▼tDissertations  Abstracts  International▼g86-12B.
■790    ▼a0181
■791    ▼aPh.D.
■792    ▼a2025
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17357469▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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