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Metallaphotoredox Catalysis Towards the Development of Late-Stage Functionalization and Cross-Coupling Methodology
Metallaphotoredox Catalysis Towards the Development of Late-Stage Functionalization and Cross-Coupling Methodology
상세정보
- 자료유형
- 학위논문 서양
- 최종처리일시
- 20260202103506
- ISBN
- 9798280747234
- DDC
- 547
- 저자명
- Mao, Edna.
- 서명/저자
- Metallaphotoredox Catalysis Towards the Development of Late-Stage Functionalization and Cross-Coupling Methodology
- 발행사항
- [Sl] : Princeton University, 2025
- 발행사항
- Ann Arbor : ProQuest Dissertations & Theses, 2025
- 형태사항
- 390 p
- 주기사항
- Source: Dissertations Abstracts International, Volume: 86-12, Section: B.
- 주기사항
- Advisor: MacMillan, David W. C.
- 학위논문주기
- Thesis (Ph.D.)--Princeton University, 2025.
- 초록/해제
- 요약The development of new catalytic methodologies for the construction of organic molecules is a central pursuit in the chemical sciences. Advancements in synthetic methods have the potential to drive progress across multiple disciplines, facilitating the discovery of new pharmaceuticals, biotechnologies, materials, and consumer goods. In recent years, visible-light-driven catalysis has emerged as a powerful strategy for enabling the efficient and selective transformation of readily available feedstocks into value-added products. By leveraging photocatalysts to mediate the controlled activation of inert functional groups, this approach provides access to reactive intermediates under mild conditions.A particularly impactful advancement in this field is the integration of photocatalysis with transition metal catalysis, a strategy known as metallaphotoredox catalysis. The ability of this dual catalytic platform to generate radical intermediates under mild conditions has provided new opportunities for late-stage functionalization (Chapters 2 & 3). Additionally, the ability to access reactive intermediates from inert organic functionality has significantly expanded the scope of bond-forming reactions and has facilitated the modular assembly of C(sp³)-rich molecular architectures from abundant precursors, including alcohols (Chapter 3) and alkenes (Chapter 4). The following chapters will explore the development and application of metallaphotoredox catalysis in these contexts, highlighting its potential to streamline complex molecule synthesis.
- 일반주제명
- Organic chemistry
- 일반주제명
- Chemistry
- 일반주제명
- Physical chemistry
- 키워드
- Cross coupling
- 기타저자
- Princeton University Chemistry
- 기본자료저록
- Dissertations Abstracts International. 86-12B.
- 전자적 위치 및 접속
- 로그인 후 원문을 볼 수 있습니다.
MARC
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■006m o d
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■020 ▼a9798280747234
■035 ▼a(MiAaPQ)AAI32002694
■040 ▼aMiAaPQ▼cMiAaPQ
■0820 ▼a547
■1001 ▼aMao, Edna.
■24510▼aMetallaphotoredox Catalysis Towards the Development of Late-Stage Functionalization and Cross-Coupling Methodology
■260 ▼a[Sl]▼bPrinceton University▼c2025
■260 1▼aAnn Arbor▼bProQuest Dissertations & Theses▼c2025
■300 ▼a390 p
■500 ▼aSource: Dissertations Abstracts International, Volume: 86-12, Section: B.
■500 ▼aAdvisor: MacMillan, David W. C.
■5021 ▼aThesis (Ph.D.)--Princeton University, 2025.
■520 ▼aThe development of new catalytic methodologies for the construction of organic molecules is a central pursuit in the chemical sciences. Advancements in synthetic methods have the potential to drive progress across multiple disciplines, facilitating the discovery of new pharmaceuticals, biotechnologies, materials, and consumer goods. In recent years, visible-light-driven catalysis has emerged as a powerful strategy for enabling the efficient and selective transformation of readily available feedstocks into value-added products. By leveraging photocatalysts to mediate the controlled activation of inert functional groups, this approach provides access to reactive intermediates under mild conditions.A particularly impactful advancement in this field is the integration of photocatalysis with transition metal catalysis, a strategy known as metallaphotoredox catalysis. The ability of this dual catalytic platform to generate radical intermediates under mild conditions has provided new opportunities for late-stage functionalization (Chapters 2 & 3). Additionally, the ability to access reactive intermediates from inert organic functionality has significantly expanded the scope of bond-forming reactions and has facilitated the modular assembly of C(sp³)-rich molecular architectures from abundant precursors, including alcohols (Chapter 3) and alkenes (Chapter 4). The following chapters will explore the development and application of metallaphotoredox catalysis in these contexts, highlighting its potential to streamline complex molecule synthesis.
■590 ▼aSchool code: 0181.
■650 4▼aOrganic chemistry
■650 4▼aChemistry
■650 4▼aPhysical chemistry
■653 ▼aCross coupling
■653 ▼aLate-stage functionalization
■653 ▼aMetallaphotoredox catalysis
■653 ▼aPhotoredox catalysis
■653 ▼aOrganic molecules
■690 ▼a0490
■690 ▼a0485
■690 ▼a0494
■71020▼aPrinceton University▼bChemistry.
■7730 ▼tDissertations Abstracts International▼g86-12B.
■790 ▼a0181
■791 ▼aPh.D.
■792 ▼a2025
■793 ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17357397▼nKERIS▼z이 자료의 원문은 한국교육학술정보원에서 제공합니다.
