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The Validation and Application of New Methods in Microplastics Research
The Validation and Application of New Methods in Microplastics Research
The Validation and Application of New Methods in Microplastics Research

상세정보

자료유형  
 학위논문 서양
최종처리일시  
20260202104833
ISBN  
9798291504079
DDC  
577
저자명  
Kosuth, Mary Song-an.
서명/저자  
The Validation and Application of New Methods in Microplastics Research
발행사항  
[Sl] : University of Minnesota, 2025
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2025
형태사항  
251 p
주기사항  
Source: Dissertations Abstracts International, Volume: 87-02, Section: B.
주기사항  
Advisor: Simcik, Matt.
학위논문주기  
Thesis (Ph.D.)--University of Minnesota, 2025.
초록/해제  
요약Plastic products subjected to natural weathering and anthropogenic activities splinter into progressively finer particles throughout their entire lifecycle. Eight decades of this material's continual degradation, combined with an ever-expanding global plastics market, results in the gradual accumulation of small (1 - 5,000 µm) synthetic particles known as microplastics. These fossil fuel-derived materials settle and flow between environmental matrices such as air, water, soil, and biota as fragments, fibers, foams, and films. While their presence is known and thoroughly documented, questions remain about the source, fate, and transport of microplastics, the human and ecological health implications, and the most effective means of constraining their planetary circulation. These questions persist, in part, because released contaminant particles are vastly heterogeneous. Their original fabrication involves an essential synthetic polymer or co-polymer resin merged with myriad chemical additives subjected to a unique set of degradative forces that may involve mechanical stress and/or distinct enzymatic and chemical conditions. In addition to these challenges, the methods applied to isolate, identify, and characterize contaminant particles are not fully standardized, making results difficult to replicate and leaving uncertainty about findings. This dissertation seeks to enhance sample processing methods for the detection, enumeration, and physical-chemical characterization of microplastic contamination for three applications: 1) fate and transport research, 2) consumer exposure research, and 3) efforts to enhance science literacy.While this work focuses on advancing laboratory processing methods for the extraction of microplastics from filtered lab water and potable tap water, they can easily extend to other environmental media such as air, raw water, and wastewater. Method enhancement centers on improving quality assurance and quality control measures and generating a comprehensive chemical and physical profile of contaminant particles. This validated method, applied to a 52-week examination of urban atmospheric fallout in a humid continental climate, elucidates particle fate and transport by comparing abundance, size, morphology, and chemical composition of microplastic contaminant particles in weather conditions that vary in terms of precipitation and temperature. Next, the improved methods are applied to a study involving the potential release of microplastics from reusable sports water bottles as they are used and cared for by members of a local cycling team over the course of 92 days. Once again, microplastic abundance, size, morphology, and chemical composition are examined to see if there are any changes linked to bottle composition and design, frequency of use, and washing habits. Finally, these verified methods are adapted for use by non-scientists in a statewide citizen science project that seeks to educate high school students about microplastic contaminants, improve overall science literacy, foster civic engagement, while generating rigorous data across a broad temporal and geographic expanse.
일반주제명  
Environmental science
일반주제명  
Polymer chemistry
일반주제명  
Toxicology
일반주제명  
Plastics
키워드  
Citizen science project
키워드  
Microplastics
키워드  
Passive air sampling
키워드  
Reusable bottles
기타저자  
University of Minnesota Environmental Health
기본자료저록  
Dissertations Abstracts International. 87-02B.
전자적 위치 및 접속  
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■1001  ▼aKosuth,  Mary  Song-an.
■24510▼aThe  Validation  and  Application  of  New  Methods  in  Microplastics  Research
■260    ▼a[Sl]▼bUniversity  of  Minnesota▼c2025
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2025
■300    ▼a251  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  87-02,  Section:  B.
■500    ▼aAdvisor:  Simcik,  Matt.
■5021  ▼aThesis  (Ph.D.)--University  of  Minnesota,  2025.
■520    ▼aPlastic  products  subjected  to  natural  weathering  and  anthropogenic  activities  splinter  into  progressively  finer  particles  throughout  their  entire  lifecycle.  Eight  decades  of  this  material's  continual  degradation,  combined  with  an  ever-expanding  global  plastics  market,  results  in  the  gradual  accumulation  of  small  (1  -  5,000  µm)  synthetic  particles  known  as  microplastics.  These  fossil  fuel-derived  materials  settle  and  flow  between  environmental  matrices  such  as  air,  water,  soil,  and  biota  as  fragments,  fibers,  foams,  and  films.  While  their  presence  is  known  and  thoroughly  documented,  questions  remain  about  the  source,  fate,  and  transport  of  microplastics,  the  human  and  ecological  health  implications,  and  the  most  effective  means  of  constraining  their  planetary  circulation.  These  questions  persist,  in  part,  because  released  contaminant  particles  are  vastly  heterogeneous.  Their  original  fabrication  involves  an  essential  synthetic  polymer  or  co-polymer  resin  merged  with  myriad  chemical  additives  subjected  to  a  unique  set  of  degradative  forces  that  may  involve  mechanical  stress  and/or  distinct  enzymatic  and  chemical  conditions.  In  addition  to  these  challenges,  the  methods  applied  to  isolate,  identify,  and  characterize  contaminant  particles  are  not  fully  standardized,  making  results  difficult  to  replicate  and  leaving  uncertainty  about  findings.  This  dissertation  seeks  to  enhance  sample  processing  methods  for  the  detection,  enumeration,  and  physical-chemical  characterization  of  microplastic  contamination  for  three  applications:  1)  fate  and  transport  research,  2)  consumer  exposure  research,  and  3)  efforts  to  enhance  science  literacy.While  this  work  focuses  on  advancing  laboratory  processing  methods  for  the  extraction  of  microplastics  from  filtered  lab  water  and  potable  tap  water,  they  can  easily  extend  to  other  environmental  media  such  as  air,  raw  water,  and  wastewater.  Method  enhancement  centers  on  improving  quality  assurance  and  quality  control  measures  and  generating  a  comprehensive  chemical  and  physical  profile  of  contaminant  particles.  This  validated  method,  applied  to  a  52-week  examination  of  urban  atmospheric  fallout  in  a  humid  continental  climate,  elucidates  particle  fate  and  transport  by  comparing  abundance,  size,  morphology,  and  chemical  composition  of  microplastic  contaminant  particles  in  weather  conditions  that  vary  in  terms  of  precipitation  and  temperature.  Next,  the  improved  methods  are  applied  to  a  study  involving  the  potential  release  of  microplastics  from  reusable  sports  water  bottles  as  they  are  used  and  cared  for  by  members  of  a  local  cycling  team  over  the  course  of  92  days.  Once  again,  microplastic  abundance,  size,  morphology,  and  chemical  composition  are  examined  to  see  if  there  are  any  changes  linked  to  bottle  composition  and  design,  frequency  of  use,  and  washing  habits.  Finally,  these  verified  methods  are  adapted  for  use  by  non-scientists  in  a  statewide  citizen  science  project  that  seeks  to  educate  high  school  students  about  microplastic  contaminants,  improve  overall  science  literacy,  foster  civic  engagement,  while  generating  rigorous  data  across  a  broad  temporal  and  geographic  expanse.
■590    ▼aSchool  code:  0130.
■650  4▼aEnvironmental  science
■650  4▼aPolymer  chemistry
■650  4▼aToxicology
■650  4▼aPlastics
■653    ▼aCitizen  science  project
■653    ▼aMicroplastics
■653    ▼aPassive  air  sampling
■653    ▼aReusable  bottles
■690    ▼a0768
■690    ▼a0795
■690    ▼a0495
■690    ▼a0383
■71020▼aUniversity  of  Minnesota▼bEnvironmental  Health.
■7730  ▼tDissertations  Abstracts  International▼g87-02B.
■790    ▼a0130
■791    ▼aPh.D.
■792    ▼a2025
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17359088▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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