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Resonant Quantum Sensing and Emission in Nanoscale Systems
Resonant Quantum Sensing and Emission in Nanoscale Systems
Resonant Quantum Sensing and Emission in Nanoscale Systems

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자료유형  
 학위논문 서양
최종처리일시  
20260202103528
ISBN  
9798288863356
DDC  
530
저자명  
Sanborn, Collin Richard.
서명/저자  
Resonant Quantum Sensing and Emission in Nanoscale Systems
발행사항  
[Sl] : University of California, Berkeley, 2025
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2025
형태사항  
105 p
주기사항  
Source: Dissertations Abstracts International, Volume: 87-01, Section: B.
주기사항  
Advisor: Wang, Feng.
학위논문주기  
Thesis (Ph.D.)--University of California, Berkeley, 2025.
초록/해제  
요약Studies of sensitive quantum systems are almost always limited by considerations of signals and noise. A crucial tool in the scientist's toolbox when approaching these systems is a strong understanding of resonant excitation, where energetic alignment between applied signals and levels in the studied system yields large increases in signal to noise ratio. This thesis explores two different nanoscale systems through this unifying approach. I will first detail the engineering of nanoscale piezoelectric resonators for high-resolution scanning probe measurements. Many atomic and subatomic resolution atomic force microcopy studies have been published in the past two decades. The probes at the heart of these studies, however, are not state-of-the-art resonators when compared to the advances in MEMS over the same period of time. Higher quality factor (Q) and operational frequency (f0) resonators confer significantly reduced noise levels and improved resolution to AFM systems. I will detail the design, simulation, fabrication, and measurement of high Q and f0 piezoelectric resonators made from LiNbO3. LiNbO3 naturally offers a great platform for such resonators with large piezoelectric coupling and acoustic velocities. These resonators achieve noise figures multiple orders of magnitude higher than existing probes for AFM and offer to greatly improve the ease of achieving subatomic resolution and high speed scanning probe measurements.I will then discuss resonances in systems of quantum single-photon emitters in monolayer tungsten diselenide (WSe2). Monolayer WSe2 has shown promise as a quantum light source due to its exciton-mediated single photon emission combined with its potential to be integrated into a variety of on-chip photonic platforms. These applications have been hampered due to a lack of understanding of the defect species involved in the single-photon emission mechanism. We use photoluminescence excitation to directly probe the energy levels associated with these defects while monitoring the quantum emission, finding that many key properties of the single-photon emission are directly affected by the excitation energy. This reveals the presence and nature of complex structures of defect levels which mediate the properties of WSe2's quantum emission. 
일반주제명  
Physics
일반주제명  
Nanotechnology
일반주제명  
Condensed matter physics
일반주제명  
Applied physics
키워드  
2D materials
키워드  
Atomic force microscopy
키워드  
Quantum systems
키워드  
Piezoelectric materials
키워드  
Single photon emitter
키워드  
Nanoscale systems
기타저자  
University of California, Berkeley Applied Science & Technology
기본자료저록  
Dissertations Abstracts International. 87-01B.
전자적 위치 및 접속  
로그인 후 원문을 볼 수 있습니다.

MARC

 008260126s2025        us                              c    eng  d
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■00520260202103528
■006m          o    d                
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■020    ▼a9798288863356
■035    ▼a(MiAaPQ)AAI32039526
■040    ▼aMiAaPQ▼cMiAaPQ
■0820  ▼a530
■1001  ▼aSanborn,  Collin  Richard.
■24510▼aResonant  Quantum  Sensing  and  Emission  in  Nanoscale  Systems
■260    ▼a[Sl]▼bUniversity  of  California,  Berkeley▼c2025
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2025
■300    ▼a105  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  87-01,  Section:  B.
■500    ▼aAdvisor:  Wang,  Feng.
■5021  ▼aThesis  (Ph.D.)--University  of  California,  Berkeley,  2025.
■520    ▼aStudies  of  sensitive  quantum  systems  are  almost  always  limited  by  considerations  of  signals  and  noise.  A  crucial  tool  in  the  scientist's  toolbox  when  approaching  these  systems  is  a  strong  understanding  of  resonant  excitation,  where  energetic  alignment  between  applied  signals  and  levels  in  the  studied  system  yields  large  increases  in  signal  to  noise  ratio.  This  thesis  explores  two  different  nanoscale  systems  through  this  unifying  approach. I  will  first  detail  the  engineering  of  nanoscale  piezoelectric  resonators  for  high-resolution  scanning  probe  measurements.  Many  atomic  and  subatomic  resolution  atomic  force  microcopy  studies  have  been  published  in  the  past  two  decades.  The  probes  at  the  heart  of  these  studies,  however,  are  not  state-of-the-art  resonators  when  compared  to  the  advances  in  MEMS  over  the  same  period  of  time.  Higher  quality  factor  (Q)  and  operational  frequency  (f0)  resonators  confer  significantly  reduced  noise  levels  and  improved  resolution  to  AFM  systems.  I  will  detail  the  design,  simulation,  fabrication,  and  measurement  of  high  Q  and  f0  piezoelectric  resonators  made  from  LiNbO3.  LiNbO3  naturally  offers  a  great  platform  for  such  resonators  with  large  piezoelectric  coupling  and  acoustic  velocities.  These  resonators  achieve  noise  figures  multiple  orders  of  magnitude  higher  than  existing  probes  for  AFM  and  offer  to  greatly  improve  the  ease  of  achieving  subatomic  resolution  and  high  speed  scanning  probe  measurements.I  will  then  discuss  resonances  in  systems  of  quantum  single-photon  emitters  in  monolayer  tungsten  diselenide  (WSe2).  Monolayer  WSe2  has  shown  promise  as  a  quantum  light  source  due  to  its  exciton-mediated  single  photon  emission  combined  with  its  potential  to  be  integrated  into  a  variety  of  on-chip  photonic  platforms.  These  applications  have  been  hampered  due  to  a  lack  of  understanding  of  the  defect  species  involved  in  the  single-photon  emission  mechanism.  We  use  photoluminescence  excitation  to  directly  probe  the  energy  levels  associated  with  these  defects  while  monitoring  the  quantum  emission,  finding  that  many  key  properties  of  the  single-photon  emission  are  directly  affected  by  the  excitation  energy.  This  reveals  the  presence  and  nature  of  complex  structures  of  defect  levels  which  mediate  the  properties  of  WSe2's  quantum  emission. 
■590    ▼aSchool  code:  0028.
■650  4▼aPhysics
■650  4▼aNanotechnology
■650  4▼aCondensed  matter  physics
■650  4▼aApplied  physics
■653    ▼a2D  materials
■653    ▼aAtomic  force  microscopy
■653    ▼aQuantum  systems
■653    ▼aPiezoelectric  materials
■653    ▼aSingle  photon  emitter
■653    ▼aNanoscale  systems
■690    ▼a0605
■690    ▼a0652
■690    ▼a0611
■690    ▼a0215
■71020▼aUniversity  of  California,  Berkeley▼bApplied  Science  &  Technology.
■7730  ▼tDissertations  Abstracts  International▼g87-01B.
■790    ▼a0028
■791    ▼aPh.D.
■792    ▼a2025
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17357551▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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