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High-Fidelity Quantum State Control of a Trapped Molecular Ion
High-Fidelity Quantum State Control of a Trapped Molecular Ion
High-Fidelity Quantum State Control of a Trapped Molecular Ion

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자료유형  
 학위논문 서양
최종처리일시  
20260202104808
ISBN  
9798291576373
DDC  
530
저자명  
Chaffee, Dalton.
서명/저자  
High-Fidelity Quantum State Control of a Trapped Molecular Ion
발행사항  
[Sl] : University of Colorado at Boulder, 2025
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2025
형태사항  
135 p
주기사항  
Source: Dissertations Abstracts International, Volume: 87-02, Section: B.
주기사항  
Advisor: Chou, Chin-wen.
학위논문주기  
Thesis (Ph.D.)--University of Colorado at Boulder, 2025.
초록/해제  
요약Ultracold molecules are a promising next-generation platform for quantum information science, precision measurement, and ultracold chemistry. However, quantum state control in molecules remains less developed than in atoms due to the added complexity from their rotational and vibrational degrees of freedom. In this thesis, I describe the development and operation of a cryogenic molecular ion-trapping experiment designed to overcome these challenges using quantum logic spectroscopy techniques. A single molecule is co-trapped with a Ca+ ion for cooling and readout, while far-detuned Raman beams are used for internal molecular state control. Cryogenically cooled radiation shields reduce the thermal radiation incident upon the trapped molecule, which can drive undesirable rovibrational transitions. The apparatus also features a molecular beam machine for loading a variety of species via resonance-enhanced multiphoton ionization. We demonstrate an unprecedented level of control of a molecule, using an adaptive Bayesian scheme to realize single-state preparation and non-destructive measurement of CaH+ with a single-state fidelity exceeding 99.4%. The demonstrated techniques are applicable to a broad class of molecular ion species, establishing a robust platform for molecular physics studies with high-fidelity molecular quantum state control.
일반주제명  
Physics
일반주제명  
Particle physics
일반주제명  
Quantum physics
키워드  
High fidelity
키워드  
Ions
키워드  
Molecules
키워드  
Rovibrational transitions
키워드  
Quantum state control
기타저자  
University of Colorado at Boulder Physics
기본자료저록  
Dissertations Abstracts International. 87-02B.
전자적 위치 및 접속  
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MARC

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■040    ▼aMiAaPQ▼cMiAaPQ
■0820  ▼a530
■1001  ▼aChaffee,  Dalton.▼0(orcid)0000-0001-8911-9486
■24510▼aHigh-Fidelity  Quantum  State  Control  of  a  Trapped  Molecular  Ion
■260    ▼a[Sl]▼bUniversity  of  Colorado  at  Boulder▼c2025
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2025
■300    ▼a135  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  87-02,  Section:  B.
■500    ▼aAdvisor:  Chou,  Chin-wen.
■5021  ▼aThesis  (Ph.D.)--University  of  Colorado  at  Boulder,  2025.
■520    ▼aUltracold  molecules  are  a  promising  next-generation  platform  for  quantum  information  science,  precision  measurement,  and  ultracold  chemistry.  However,  quantum  state  control  in  molecules  remains  less  developed  than  in  atoms  due  to  the  added  complexity  from  their  rotational  and  vibrational  degrees  of  freedom.  In  this  thesis,  I  describe  the  development  and  operation  of  a  cryogenic  molecular  ion-trapping  experiment  designed  to  overcome  these  challenges  using  quantum  logic  spectroscopy  techniques.  A  single  molecule  is  co-trapped  with  a  Ca+  ion  for  cooling  and  readout,  while  far-detuned  Raman  beams  are  used  for  internal  molecular  state  control.  Cryogenically  cooled  radiation  shields  reduce  the  thermal  radiation  incident  upon  the  trapped  molecule,  which  can  drive  undesirable  rovibrational  transitions.  The  apparatus  also  features  a  molecular  beam  machine  for  loading  a  variety  of  species  via  resonance-enhanced  multiphoton  ionization.  We  demonstrate  an  unprecedented  level  of  control  of  a  molecule,  using  an  adaptive  Bayesian  scheme  to  realize  single-state  preparation  and  non-destructive  measurement  of  CaH+  with  a  single-state  fidelity  exceeding  99.4%.  The  demonstrated  techniques  are  applicable  to  a  broad  class  of  molecular  ion  species,  establishing  a  robust  platform  for  molecular  physics  studies  with  high-fidelity  molecular  quantum  state  control.
■590    ▼aSchool  code:  0051.
■650  4▼aPhysics
■650  4▼aParticle  physics
■650  4▼aQuantum  physics
■653    ▼aHigh  fidelity
■653    ▼aIons
■653    ▼aMolecules
■653    ▼aRovibrational  transitions
■653    ▼aQuantum  state  control
■690    ▼a0605
■690    ▼a0798
■690    ▼a0599
■71020▼aUniversity  of  Colorado  at  Boulder▼bPhysics.
■7730  ▼tDissertations  Abstracts  International▼g87-02B.
■790    ▼a0051
■791    ▼aPh.D.
■792    ▼a2025
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17358904▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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