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Charge Density Wave Dynamics in Transition Metal Dichalcogenides Probed with Ultrafast Electron Diffraction and X-Ray Photon Correlation Spectroscopy
Charge Density Wave Dynamics in Transition Metal Dichalcogenides Probed with Ultrafast Ele...
Charge Density Wave Dynamics in Transition Metal Dichalcogenides Probed with Ultrafast Electron Diffraction and X-Ray Photon Correlation Spectroscopy

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자료유형  
 학위논문 서양
최종처리일시  
20260202105419
ISBN  
9798297684997
DDC  
530
저자명  
Sutter, Thomas M.
서명/저자  
Charge Density Wave Dynamics in Transition Metal Dichalcogenides Probed with Ultrafast Electron Diffraction and X-Ray Photon Correlation Spectroscopy
발행사항  
[Sl] : University of California, Los Angeles, 2025
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2025
형태사항  
213 p
주기사항  
Source: Dissertations Abstracts International, Volume: 87-04, Section: B.
주기사항  
Advisor: Kogar, Anshul.
학위논문주기  
Thesis (Ph.D.)--University of California, Los Angeles, 2025.
초록/해제  
요약Charge density waves (CDWs) are electronic modulations that occur at low temperature in many crystalline materials; they underlie fascinating dynamic behaviors such as collective sliding transport and narrow-band noise, and engage in various interactions with superconductivity. CDWs can be dynamically manipulated with light, opening new possibilities for materials control and the realization of hidden non-equilibrium phases. This dissertation investigates CDW dynamics using ultrafast electron diffraction (UED) and X-ray photon correlation spectroscopy (XPCS). A UED beamline with sub-picosecond time resolution was developed for this purpose. Using this instrument, UED experiments reveal a light-induced topological transition to a hidden liquid CDW phase in 1T-TaS2 and a coupling between CDW order and a shear structural instability in VTe2. XPCS measurements of Cu-intercalated 1T-TiSe2 uncover slow phase-fluctuation dynamics that drive the system into a metastable, short-range ordered state coexisting with superconductivity. Together, these studies demonstrate the rich non-equilibrium behavior of CDWs and the utility of time-resolved techniques in uncovering their dynamics.
일반주제명  
Condensed matter physics
일반주제명  
Applied physics
일반주제명  
Materials science
일반주제명  
Optics
키워드  
Charge density waves
키워드  
Light-induced dynamics
키워드  
Transition metal dichalcogenides
키워드  
Ultrafast electron diffraction
키워드  
X-ray photon correlation spectroscopy
기타저자  
University of California, Los Angeles Physics 0666
기본자료저록  
Dissertations Abstracts International. 87-04B.
전자적 위치 및 접속  
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■006m          o    d                
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■020    ▼a9798297684997
■035    ▼a(MiAaPQ)AAI32278365
■040    ▼aMiAaPQ▼cMiAaPQ
■0820  ▼a530
■1001  ▼aSutter,  Thomas  M.
■24510▼aCharge  Density  Wave  Dynamics  in  Transition  Metal  Dichalcogenides  Probed  with  Ultrafast  Electron  Diffraction  and  X-Ray  Photon  Correlation  Spectroscopy
■260    ▼a[Sl]▼bUniversity  of  California,  Los  Angeles▼c2025
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2025
■300    ▼a213  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  87-04,  Section:  B.
■500    ▼aAdvisor:  Kogar,  Anshul.
■5021  ▼aThesis  (Ph.D.)--University  of  California,  Los  Angeles,  2025.
■520    ▼aCharge  density  waves  (CDWs)  are  electronic  modulations  that  occur  at  low  temperature  in  many  crystalline  materials;  they  underlie  fascinating  dynamic  behaviors  such  as  collective  sliding  transport  and  narrow-band  noise,  and  engage  in  various  interactions  with  superconductivity.  CDWs  can  be  dynamically  manipulated  with  light,  opening  new  possibilities  for  materials  control  and  the  realization  of  hidden  non-equilibrium  phases.  This  dissertation  investigates  CDW  dynamics  using  ultrafast  electron  diffraction  (UED)  and  X-ray  photon  correlation  spectroscopy  (XPCS).  A  UED  beamline  with  sub-picosecond  time  resolution  was  developed  for  this  purpose.  Using  this  instrument,  UED  experiments  reveal  a  light-induced  topological  transition  to  a  hidden  liquid  CDW  phase  in  1T-TaS2  and  a  coupling  between  CDW  order  and  a  shear  structural  instability  in  VTe2.  XPCS  measurements  of  Cu-intercalated  1T-TiSe2  uncover  slow  phase-fluctuation  dynamics  that  drive  the  system  into  a  metastable,  short-range  ordered  state  coexisting  with  superconductivity.  Together,  these  studies  demonstrate  the  rich  non-equilibrium  behavior  of  CDWs  and  the  utility  of  time-resolved  techniques  in  uncovering  their  dynamics.
■590    ▼aSchool  code:  0031.
■650  4▼aCondensed  matter  physics
■650  4▼aApplied  physics
■650  4▼aMaterials  science
■650  4▼aOptics
■653    ▼aCharge  density  waves
■653    ▼aLight-induced  dynamics
■653    ▼aTransition  metal  dichalcogenides
■653    ▼aUltrafast  electron  diffraction
■653    ▼aX-ray  photon  correlation  spectroscopy
■690    ▼a0611
■690    ▼a0752
■690    ▼a0794
■690    ▼a0215
■71020▼aUniversity  of  California,  Los  Angeles▼bPhysics  0666.
■7730  ▼tDissertations  Abstracts  International▼g87-04B.
■790    ▼a0031
■791    ▼aPh.D.
■792    ▼a2025
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17360286▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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