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Spectroscopy of Strongly Correlated Emergent Phases in Unconventional Insulators and Superconductors
Spectroscopy of Strongly Correlated Emergent Phases in Unconventional Insulators and Super...
Spectroscopy of Strongly Correlated Emergent Phases in Unconventional Insulators and Superconductors

상세정보

자료유형  
 학위논문 서양
최종처리일시  
20260202104736
ISBN  
9798290648750
DDC  
530
저자명  
Xu, Kejun.
서명/저자  
Spectroscopy of Strongly Correlated Emergent Phases in Unconventional Insulators and Superconductors
발행사항  
[Sl] : Stanford University, 2024
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2024
형태사항  
168 p
주기사항  
Source: Dissertations Abstracts International, Volume: 87-01, Section: B.
주기사항  
Advisor: Shen, Zhi-Xun.
학위논문주기  
Thesis (Ph.D.)--Stanford University, 2024.
초록/해제  
요약Correlated electron systems is a central topic in modern condensed matter physics, both due to the profound significance of emergent phases as well as their potential for technological applications. To harness the power of these materials that reside deeply in the quantum regime, we must first understand the connection between macroscopic properties and microscopic mechanisms. The difficulty with strongly correlated electron systems is that they are usually described by a strongly entangled many-body state, which precludes their understanding by the traditional tools of perturbation theory. This renders experimental measurements all the more important, as we may find many surprises that could not yet be predicted from first principles. One powerful probing tool at the disposal of experimental condensed matter physicists is angle-resolved photoemission spectroscopy (ARPES), which measures the energy and momentum of electrons within a crystalline material. More importantly, in the context of studying correlated electron systems, ARPES affords the capability to measure interaction effects and order parameters of gapped phases. This dissertation will utilize the ARPES technique to investigate two kinds of correlated electron systems: an unconventional cuprate superconductor Nd2-xCexCuO4(NCCO) and an unusual correlated insulator FeSb2.In the first portion of this dissertation, I will detail systematic ARPES studies of a prototypical n-type cuprate NCCO. These investigations begin near the optimally doped regime near x = 0.15 with the highest superconducting transition temperatures (Tc). By measuring the Bogoliubov quasiparticle peak with ARPES for the first time in the n-type cuprates, we show the existence and importance of a set of "gossamer" Fermi surface states within the energy gap imparted by antiferromagnetism. This result reveal that the single low energy band is fragmented into two sectors of states in the n-type cuprates: one sector reconstructed by the antiferromagnetism provides the pairing interactions and one sector of residual states hosts the paired quasiparticles. Furthermore, we find an unusual form of coupling between the antiferromagnetism and phonons in the form of a replica band copying the dispersion of the antiferromagnetically reconstructed states, highlighting the importance of the lattice involvement in shaping the low energy electronic structure. Moving away from the optimal doped regime, we discover an anomalous normal state gap in underdoped NCCO that is inconsistent with known orders and fluctuations. Instead, this anomalous gap is attributed to a state with incoherent pairs, raising the prospect of engineering much higher Tcin these materials.In the second portion of this dissertation, I will explore the interplay between topology and correlations in the candidate topological Kondo insulator FeSb2. This material is a rare example of a 3d-electron-based correlated insulator exhibiting Kondo lattice behavior, which usually arises from 4felectron systems. Starting from transport investigations of a low temperature resistivity anomaly indicative of surface conduction, I will present spectroscopic evidence for a rich set of surface states that underlie the low temperature transport. Furthermore, I will discuss the observation of anomalous quantum oscillations in high-magnetic-field torque magnetometry measurements, which indicates the existence of unconventional magnetism and Landau quantization in a bulk insulator. Our results pave the way for further comparative studies of 3dand 4fKondo insulators that exhibit unconventional insulating behaviors.
일반주제명  
Phase transitions
일반주제명  
Heat
일반주제명  
Physics
일반주제명  
Energy
일반주제명  
Electrons
일반주제명  
Superconductivity
일반주제명  
Spectrum analysis
일반주제명  
Crystals
기타저자  
Stanford University.
기본자료저록  
Dissertations Abstracts International. 87-01B.
전자적 위치 및 접속  
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MARC

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■0820  ▼a530
■1001  ▼aXu,  Kejun.
■24510▼aSpectroscopy  of  Strongly  Correlated  Emergent  Phases  in  Unconventional  Insulators  and  Superconductors
■260    ▼a[Sl]▼bStanford  University▼c2024
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2024
■300    ▼a168  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  87-01,  Section:  B.
■500    ▼aAdvisor:  Shen,  Zhi-Xun.
■5021  ▼aThesis  (Ph.D.)--Stanford  University,  2024.
■520    ▼aCorrelated  electron  systems  is  a  central  topic  in  modern  condensed  matter  physics,  both  due  to  the  profound  significance  of  emergent  phases  as  well  as  their  potential  for  technological  applications.  To  harness  the  power  of  these  materials  that  reside  deeply  in  the  quantum  regime,  we  must  first  understand  the  connection  between  macroscopic  properties  and  microscopic  mechanisms.  The  difficulty  with  strongly  correlated  electron  systems  is  that  they  are  usually  described  by  a  strongly  entangled  many-body  state,  which  precludes  their  understanding  by  the  traditional  tools  of  perturbation  theory.  This  renders  experimental  measurements  all  the  more  important,  as  we  may  find  many  surprises  that  could  not  yet  be  predicted  from  first  principles.  One  powerful  probing  tool  at  the  disposal  of  experimental  condensed  matter  physicists  is  angle-resolved  photoemission  spectroscopy  (ARPES),  which  measures  the  energy  and  momentum  of  electrons  within  a  crystalline  material.  More  importantly,  in  the  context  of  studying  correlated  electron  systems,  ARPES  affords  the  capability  to  measure  interaction  effects  and  order  parameters  of  gapped  phases.  This  dissertation  will  utilize  the  ARPES  technique  to  investigate  two  kinds  of  correlated  electron  systems:  an  unconventional  cuprate  superconductor  Nd2-xCexCuO4(NCCO)  and  an  unusual  correlated  insulator  FeSb2.In  the  first  portion  of  this  dissertation,  I  will  detail  systematic  ARPES  studies  of  a  prototypical  n-type  cuprate  NCCO.  These  investigations  begin  near  the  optimally  doped  regime  near  x  =  0.15  with  the  highest  superconducting  transition  temperatures  (Tc).  By  measuring  the  Bogoliubov  quasiparticle  peak  with  ARPES  for  the  first  time  in  the  n-type  cuprates,  we  show  the  existence  and  importance  of  a  set  of  "gossamer"  Fermi  surface  states  within  the  energy  gap  imparted  by  antiferromagnetism.  This  result  reveal  that  the  single  low  energy  band  is  fragmented  into  two  sectors  of  states  in  the  n-type  cuprates:  one  sector  reconstructed  by  the  antiferromagnetism  provides  the  pairing  interactions  and  one  sector  of  residual  states  hosts  the  paired  quasiparticles.  Furthermore,  we  find  an  unusual  form  of  coupling  between  the  antiferromagnetism  and  phonons  in  the  form  of  a  replica  band  copying  the  dispersion  of  the  antiferromagnetically  reconstructed  states,  highlighting  the  importance  of  the  lattice  involvement  in  shaping  the  low  energy  electronic  structure.  Moving  away  from  the  optimal  doped  regime,  we  discover  an  anomalous  normal  state  gap  in  underdoped  NCCO  that  is  inconsistent  with  known  orders  and  fluctuations.  Instead,  this  anomalous  gap  is  attributed  to  a  state  with  incoherent  pairs,  raising  the  prospect  of  engineering  much  higher  Tcin  these  materials.In  the  second  portion  of  this  dissertation,  I  will  explore  the  interplay  between  topology  and  correlations  in  the  candidate  topological  Kondo  insulator  FeSb2.  This  material  is  a  rare  example  of  a  3d-electron-based  correlated  insulator  exhibiting  Kondo  lattice  behavior,  which  usually  arises  from  4felectron  systems.  Starting  from  transport  investigations  of  a  low  temperature  resistivity  anomaly  indicative  of  surface  conduction,  I  will  present  spectroscopic  evidence  for  a  rich  set  of  surface  states  that  underlie  the  low  temperature  transport.  Furthermore,  I  will  discuss  the  observation  of  anomalous  quantum  oscillations  in  high-magnetic-field  torque  magnetometry  measurements,  which  indicates  the  existence  of  unconventional  magnetism  and  Landau  quantization  in  a  bulk  insulator.  Our  results  pave  the  way  for  further  comparative  studies  of  3dand  4fKondo  insulators  that  exhibit  unconventional  insulating  behaviors.
■590    ▼aSchool  code:  0212.
■650  4▼aPhase  transitions
■650  4▼aHeat
■650  4▼aPhysics
■650  4▼aEnergy
■650  4▼aElectrons
■650  4▼aSuperconductivity
■650  4▼aSpectrum  analysis
■650  4▼aCrystals
■690    ▼a0605
■690    ▼a0791
■71020▼aStanford  University.
■7730  ▼tDissertations  Abstracts  International▼g87-01B.
■790    ▼a0212
■791    ▼aPh.D.
■792    ▼a2024
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17358678▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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