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Thermodynamics of Interacting Electrons in Two-Dimensional Semiconductor Homostructures
Thermodynamics of Interacting Electrons in Two-Dimensional Semiconductor Homostructures
Thermodynamics of Interacting Electrons in Two-Dimensional Semiconductor Homostructures

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자료유형  
 학위논문 서양
최종처리일시  
20260202104737
ISBN  
9798290652771
DDC  
530
저자명  
Foutty, Benjamin Aaron.
서명/저자  
Thermodynamics of Interacting Electrons in Two-Dimensional Semiconductor Homostructures
발행사항  
[Sl] : Stanford University, 2025
발행사항  
Ann Arbor : ProQuest Dissertations & Theses, 2025
형태사항  
202 p
주기사항  
Source: Dissertations Abstracts International, Volume: 87-01, Section: B.
주기사항  
Advisor: Feldman, Ben.
학위논문주기  
Thesis (Ph.D.)--Stanford University, 2025.
초록/해제  
요약Semiconductor moire materials, in which atomically-thin, two-dimensional sheets of semi-conductors are twisted and stacked together, have emerged as an ideal platform to study the interplay of magnetism, topology, and electronic correlations. Semiconductor homostruc-tures, where the moire interface is composed of the same atomic components, are a partic-ularly tunable subset of these materials by enabling long moire wavelengths and relatively stronger electronic interactions at low twist angles. Due to challenges of angular disorder in these systems, they have been difficult to examine using measurements that average spatially over devices. In this thesis, I will describe a set of experiments using scanning single electron transistor (SET) microscopy to explore the resulting thermodynamic ground states and charged excitations of interacting carriers in these systems with 100 nm spatial resolution.First, I motivate scanning SET as a well-suited probe of these twisted semiconductors. Then, I describe measurements via scanning SET on the the effects of interactions on the integer quantum Hall limit in monolayer WSe₂, a transition metal dichalcogenide (TMD) semiconductor that will form the basic building block of the rest of the devices studied in this thesis. Moving to twisted bilayer WSe2(tWSe₂), I present findings of multiple Chern insulating states at zero magnetic field, providing the first evidence of topological electronic bands in these systems. We are also able to control these topological phases by driving a topological-to-trivial phase transition as a function of a locally applied electric field using the SET tip. I also examine the thermodynamics of tWSe2, in a large magnetic field, in which the combination of a large Zeeman energy and Hofstadter's butterfly physics leads to a cascade of magnetic phase transitions. These transitions shed light on the spin-resolved Hofstadter spectrum and can help to disentangle the role of material and moire effects on the nature of the correlated ground states.Beyond tWSe2, I show data on twisted double bilayers (tdWSe2) and twisted mono-tetralayer (t1+4WSe2) WSe2, in which the thicker structures favor valence moire bands localized at the F-valley, rather than the K-valley bands stabilized in tWSe2. In tdWSe2. I present evidence for nontrivial spin excitations driven by kinetic magnetism, as well as competition between states at the - and K-valleys. Finally, I discuss ongoing efforts to combine tunable displacement fields with scanning SET by measuring a tWSe₂ device fabricated with a monolayer graphene top gate, enabling measurements of the correlated insulating gaps in that system as a function of displacement field.
일반주제명  
Phase transitions
일반주제명  
Motivation
일반주제명  
Physics
일반주제명  
Electrons
일반주제명  
Magnetic fields
일반주제명  
Electric fields
일반주제명  
Volleyball
기타저자  
Stanford University.
기본자료저록  
Dissertations Abstracts International. 87-01B.
전자적 위치 및 접속  
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MARC

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■040    ▼aMiAaPQ▼cMiAaPQ
■0820  ▼a530
■1001  ▼aFoutty,  Benjamin  Aaron.
■24510▼aThermodynamics  of  Interacting  Electrons  in  Two-Dimensional  Semiconductor  Homostructures
■260    ▼a[Sl]▼bStanford  University▼c2025
■260  1▼aAnn  Arbor▼bProQuest  Dissertations  &  Theses▼c2025
■300    ▼a202  p
■500    ▼aSource:  Dissertations  Abstracts  International,  Volume:  87-01,  Section:  B.
■500    ▼aAdvisor:  Feldman,  Ben.
■5021  ▼aThesis  (Ph.D.)--Stanford  University,  2025.
■520    ▼aSemiconductor  moire  materials,  in  which  atomically-thin,  two-dimensional  sheets  of  semi-conductors  are  twisted  and  stacked  together,  have  emerged  as  an  ideal  platform  to  study  the  interplay  of  magnetism,  topology,  and  electronic  correlations.  Semiconductor  homostruc-tures,  where  the  moire  interface  is  composed  of  the  same  atomic  components,  are  a  partic-ularly  tunable  subset  of  these  materials  by  enabling  long  moire  wavelengths  and  relatively  stronger  electronic  interactions  at  low  twist  angles.  Due  to  challenges  of  angular  disorder  in  these  systems,  they  have  been  difficult  to  examine  using  measurements  that  average  spatially  over  devices.  In  this  thesis,  I  will  describe  a  set  of  experiments  using  scanning  single  electron  transistor  (SET)  microscopy  to  explore  the  resulting  thermodynamic  ground  states  and  charged  excitations  of  interacting  carriers  in  these  systems  with  100  nm  spatial  resolution.First,  I  motivate  scanning  SET  as  a  well-suited  probe  of  these  twisted  semiconductors.  Then,  I  describe  measurements  via  scanning  SET  on  the  the  effects  of  interactions  on  the  integer  quantum  Hall  limit  in  monolayer  WSe₂,  a  transition  metal  dichalcogenide  (TMD)  semiconductor  that  will  form  the  basic  building  block  of  the  rest  of  the  devices  studied  in  this  thesis.  Moving  to  twisted  bilayer  WSe2(tWSe₂),  I  present  findings  of  multiple  Chern  insulating  states  at  zero  magnetic  field,  providing  the  first  evidence  of  topological  electronic  bands  in  these  systems.  We  are  also  able  to  control  these  topological  phases  by  driving  a  topological-to-trivial  phase  transition  as  a  function  of  a  locally  applied  electric  field  using  the  SET  tip.  I  also  examine  the  thermodynamics  of  tWSe2,  in  a  large  magnetic  field,  in  which  the  combination  of  a  large  Zeeman  energy  and  Hofstadter's  butterfly  physics  leads  to  a  cascade  of  magnetic  phase  transitions.  These  transitions  shed  light  on  the  spin-resolved  Hofstadter  spectrum  and  can  help  to  disentangle  the  role  of  material  and  moire  effects  on  the  nature  of  the  correlated  ground  states.Beyond  tWSe2,  I  show  data  on  twisted  double  bilayers  (tdWSe2)  and  twisted  mono-tetralayer  (t1+4WSe2)  WSe2,  in  which  the  thicker  structures  favor  valence  moire  bands  localized  at  the  F-valley,  rather  than  the  K-valley  bands  stabilized  in  tWSe2.  In  tdWSe2.  I  present  evidence  for  nontrivial  spin  excitations  driven  by  kinetic  magnetism,  as  well  as  competition  between  states  at  the  -  and  K-valleys.  Finally,  I  discuss  ongoing  efforts  to  combine  tunable  displacement  fields  with  scanning  SET  by  measuring  a  tWSe₂  device  fabricated  with  a  monolayer  graphene  top  gate,  enabling  measurements  of  the  correlated  insulating  gaps  in  that  system  as  a  function  of  displacement  field.
■590    ▼aSchool  code:  0212.
■650  4▼aPhase  transitions
■650  4▼aMotivation
■650  4▼aPhysics
■650  4▼aElectrons
■650  4▼aMagnetic  fields
■650  4▼aElectric  fields
■650  4▼aVolleyball
■690    ▼a0605
■71020▼aStanford  University.
■7730  ▼tDissertations  Abstracts  International▼g87-01B.
■790    ▼a0212
■791    ▼aPh.D.
■792    ▼a2025
■793    ▼aEnglish
■85640▼uhttp://www.riss.kr/pdu/ddodLink.do?id=T17358685▼nKERIS▼z이  자료의  원문은  한국교육학술정보원에서  제공합니다.

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